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- Title
- High hardness in the biocompatible intermetallic compound β-Ti3Au.
- Creator
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Svanidze, Eteri, Besara, Tiglet, Ozaydin, M Fevsi, Tiwary, Chandra Sekhar, Wang, Jiakui K, Radhakrishnan, Sruthi, Mani, Sendurai, Xin, Yan, Han, Ke, Liang, Hong, Siegrist, Theo,...
Show moreSvanidze, Eteri, Besara, Tiglet, Ozaydin, M Fevsi, Tiwary, Chandra Sekhar, Wang, Jiakui K, Radhakrishnan, Sruthi, Mani, Sendurai, Xin, Yan, Han, Ke, Liang, Hong, Siegrist, Theo, Ajayan, Pulickel M, Morosan, E
Show less - Abstract/Description
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The search for new hard materials is often challenging, but strongly motivated by the vast application potential such materials hold. Ti3Au exhibits high hardness values (about four times those of pure Ti and most steel alloys), reduced coefficient of friction and wear rates, and biocompatibility, all of which are optimal traits for orthopedic, dental, and prosthetic applications. In addition, the ability of this compound to adhere to ceramic parts can reduce both the weight and the cost of...
Show moreThe search for new hard materials is often challenging, but strongly motivated by the vast application potential such materials hold. Ti3Au exhibits high hardness values (about four times those of pure Ti and most steel alloys), reduced coefficient of friction and wear rates, and biocompatibility, all of which are optimal traits for orthopedic, dental, and prosthetic applications. In addition, the ability of this compound to adhere to ceramic parts can reduce both the weight and the cost of medical components. The fourfold increase in the hardness of Ti3Au compared to other Ti-Au alloys and compounds can be attributed to the elevated valence electron density, the reduced bond length, and the pseudogap formation. Understanding the origin of hardness in this intermetallic compound provides an avenue toward designing superior biocompatible, hard materials.
Show less - Date Issued
- 2016-07-20
- Identifier
- FSU_pmch_27453942, 10.1126/sciadv.1600319, PMC4956191, 27453942, 27453942, 1600319
- Format
- Citation
- Title
- Nearly massless Dirac fermions hosted by Sb square net in BaMnSb2.
- Creator
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Liu, Jinyu, Hu, Jin, Cao, Huibo, Zhu, Yanglin, Chuang, Alyssa, Graf, D, Adams, D J, Radmanesh, S M A, Spinu, L, Chiorescu, I, Mao, Zhiqiang
- Abstract/Description
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Layered compounds AMnBi2 (A = Ca, Sr, Ba, or rare earth element) have been established as Dirac materials. Dirac electrons generated by the two-dimensional (2D) Bi square net in these materials are normally massive due to the presence of a spin-orbital coupling (SOC) induced gap at Dirac nodes. Here we report that the Sb square net in an isostructural compound BaMnSb2 can host nearly massless Dirac fermions. We observed strong Shubnikov-de Haas (SdH) oscillations in this material. From the...
Show moreLayered compounds AMnBi2 (A = Ca, Sr, Ba, or rare earth element) have been established as Dirac materials. Dirac electrons generated by the two-dimensional (2D) Bi square net in these materials are normally massive due to the presence of a spin-orbital coupling (SOC) induced gap at Dirac nodes. Here we report that the Sb square net in an isostructural compound BaMnSb2 can host nearly massless Dirac fermions. We observed strong Shubnikov-de Haas (SdH) oscillations in this material. From the analyses of the SdH oscillations, we find key signatures of Dirac fermions, including light effective mass (~0.052m0; m0, mass of free electron), high quantum mobility (1280 cm(2)V(-1)S(-1)) and a π Berry phase accumulated along cyclotron orbit. Compared with AMnBi2, BaMnSb2 also exhibits much more significant quasi two-dimensional (2D) electronic structure, with the out-of-plane transport showing nonmetallic conduction below 120 K and the ratio of the out-of-plane and in-plane resistivity reaching ~670. Additionally, BaMnSb2 also exhibits a G-type antiferromagnetic order below 283 K. The combination of nearly massless Dirac fermions on quasi-2D planes with a magnetic order makes BaMnSb2 an intriguing platform for seeking novel exotic phenomena of massless Dirac electrons.
Show less - Date Issued
- 2016-07-28
- Identifier
- FSU_pmch_27466151, 10.1038/srep30525, PMC4964361, 27466151, 27466151, srep30525
- Format
- Citation
- Title
- Influence of grain boundary characteristics on thermal stability in nanotwinned copper.
- Creator
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Niu, Rongmei, Han, Ke, Su, Yi-Feng, Besara, Tiglet, Siegrist, Theo M, Zuo, Xiaowei
- Abstract/Description
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High density grain boundaries provide high strength, but may introduce undesirable features, such as high Fermi levels and instability. We investigated the kinetics of recovery and recrystallization of Cu that was manufactured to include both nanotwins (NT) and high-angle columnar boundaries. We used the isothermal Johnson-Mehl-Avrami-Kolmogorov (JMAK) model to estimate activation energy values for recovery and recrystallization and compared those to values derived using the non-isothermal...
Show moreHigh density grain boundaries provide high strength, but may introduce undesirable features, such as high Fermi levels and instability. We investigated the kinetics of recovery and recrystallization of Cu that was manufactured to include both nanotwins (NT) and high-angle columnar boundaries. We used the isothermal Johnson-Mehl-Avrami-Kolmogorov (JMAK) model to estimate activation energy values for recovery and recrystallization and compared those to values derived using the non-isothermal Kissinger equation. The JMAK model hinges on an exponent that expresses the growth mechanism of a material. The exponent for this Cu was close to 0.5, indicating low-dimensional microstructure evolution, which is associated with anisotropic twin coarsening, heterogeneous recrystallization, and high stability. Since this Cu was of high purity, there was a negligible impurity-drag-effect on boundaries. The twin coarsening and heterogeneous recrystallization resulted from migration of high-angle columnar boundaries with their triple junctions in one direction, assisted by the presence of high concentration vacancies at boundaries. Analyses performed by electron energy loss spectroscopy of atomic columns at twin boundaries (TBs) and in the interior showed similar plasma peak shapes and L3 edge positions. This implies that values for conductivity and Fermi level are equal for atoms at TBs and in the interior.
Show less - Date Issued
- 2016-08-12
- Identifier
- FSU_pmch_27514474, 10.1038/srep31410, PMC4981844, 27514474, 27514474, srep31410
- Format
- Citation
- Title
- Sliding of centrosome-unattached microtubules defines key features of neuronal phenotype.
- Creator
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Rao, Anand N, Falnikar, Aditi, O'Toole, Eileen T, Morphew, Mary K, Hoenger, Andreas, Davidson, Michael W, Yuan, Xiaobing, Baas, Peter W
- Abstract/Description
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Contemporary models for neuronal migration are grounded in the view that virtually all functionally relevant microtubules (MTs) in migrating neurons are attached to the centrosome, which occupies a position between the nucleus and a short leading process. It is assumed that MTs do not undergo independent movements but rather transduce forces that enable movements of the centrosome and nucleus. The present results demonstrate that although this is mostly true, a small fraction of the MTs are...
Show moreContemporary models for neuronal migration are grounded in the view that virtually all functionally relevant microtubules (MTs) in migrating neurons are attached to the centrosome, which occupies a position between the nucleus and a short leading process. It is assumed that MTs do not undergo independent movements but rather transduce forces that enable movements of the centrosome and nucleus. The present results demonstrate that although this is mostly true, a small fraction of the MTs are centrosome-unattached, and this permits limited sliding of MTs. When this sliding is pharmacologically inhibited, the leading process becomes shorter, migration of the neuron deviates from its normal path, and the MTs within the leading process become buckled. Partial depletion of ninein, a protein that attaches MTs to the centrosome, leads to greater numbers of centrosome-unattached MTs as well as greater sliding of MTs. Concomitantly, the soma becomes less mobile and the leading process acquires an elongated morphology akin to an axon.
Show less - Date Issued
- 2016-05-09
- Identifier
- FSU_pmch_27138250, 10.1083/jcb.201506140, PMC4862329, 27138250, 27138250, jcb.201506140
- Format
- Citation
- Title
- Pressure and high-Tc superconductivity in sulfur hydrides.
- Creator
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Gor'kov, Lev P, Kresin, Vladimir Z
- Abstract/Description
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The paper discusses fundamentals of record-TC superconductivity discovered under high pressure in sulfur hydride. The rapid increase of TC with pressure in the vicinity of Pcr ≈ 123GPa is interpreted as the fingerprint of a first-order structural transition. Based on the cubic symmetry of the high-TC phase, it is argued that the lower-TC phase has a different periodicity, possibly related to an instability with a commensurate structural vector. In addition to the acoustic branches, the phonon...
Show moreThe paper discusses fundamentals of record-TC superconductivity discovered under high pressure in sulfur hydride. The rapid increase of TC with pressure in the vicinity of Pcr ≈ 123GPa is interpreted as the fingerprint of a first-order structural transition. Based on the cubic symmetry of the high-TC phase, it is argued that the lower-TC phase has a different periodicity, possibly related to an instability with a commensurate structural vector. In addition to the acoustic branches, the phonon spectrum of H3S contains hydrogen modes with much higher frequencies. Because of the complex spectrum, usual methods of calculating TC are here inapplicable. A modified approach is formulated and shown to provide realistic values for TC and to determine the relative contributions of optical and acoustic branches. The isotope effect (change of TC upon Deuterium for Hydrogen substitution) originates from high frequency phonons and differs in the two phases. The decrease of TC following its maximum in the high-TC phase is a sign of intermixing with pairing at hole-like pockets which arise in the energy spectrum of the cubic phase at the structural transition. On-pockets pairing leads to the appearance of a second gap and is remarkable for its non-adiabatic regime: hydrogen mode frequencies are comparable to the Fermi energy.
Show less - Date Issued
- 2016-05-11
- Identifier
- FSU_pmch_27167334, 10.1038/srep25608, PMC4863257, 27167334, 27167334, srep25608
- Format
- Citation
- Title
- Crystallization of spin superlattices with pressure and field in the layered magnet SrCu2(BO3)2.
- Creator
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Haravifard, S, Graf, D, Feiguin, A E, Batista, C D, Lang, J C, Silevitch, D M, Srajer, G, Gaulin, B D, Dabkowska, H A, Rosenbaum, T F
- Abstract/Description
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An exact mapping between quantum spins and boson gases provides fresh approaches to the creation of quantum condensates and crystals. Here we report on magnetization measurements on the dimerized quantum magnet SrCu2(BO3)2 at cryogenic temperatures and through a quantum-phase transition that demonstrate the emergence of fractionally filled bosonic crystals in mesoscopic patterns, specified by a sequence of magnetization plateaus. We apply tens of Teslas of magnetic field to tune the density...
Show moreAn exact mapping between quantum spins and boson gases provides fresh approaches to the creation of quantum condensates and crystals. Here we report on magnetization measurements on the dimerized quantum magnet SrCu2(BO3)2 at cryogenic temperatures and through a quantum-phase transition that demonstrate the emergence of fractionally filled bosonic crystals in mesoscopic patterns, specified by a sequence of magnetization plateaus. We apply tens of Teslas of magnetic field to tune the density of bosons and gigapascals of hydrostatic pressure to regulate the underlying interactions. Simulations help parse the balance between energy and geometry in the emergent spin superlattices. The magnetic crystallites are the end result of a progression from a direct product of singlet states in each short dimer at zero field to preferred filling fractions of spin-triplet bosons in each dimer at large magnetic field, enriching the known possibilities for collective states in both quantum spin and atomic systems.
Show less - Date Issued
- 2016-06-20
- Identifier
- FSU_pmch_27320787, 10.1038/ncomms11956, PMC4915149, 27320787, 27320787, ncomms11956
- Format
- Citation
- Title
- Label-Free Relative Quantitation of Isobaric and Isomeric Human Histone H2A and H2B Variants by Fourier Transform Ion Cyclotron Resonance Top-Down MS/MS.
- Creator
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Dang, Xibei, Singh, Amar, Spetman, Brian D, Nolan, Krystal D, Isaacs, Jennifer S, Dennis, Jonathan H, Dalton, Stephen, Marshall, Alan G, Young, Nicolas L
- Abstract/Description
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Histone variants are known to play a central role in genome regulation and maintenance. However, many variants are inaccessible by antibody-based methods or bottom-up tandem mass spectrometry due to their highly similar sequences. For many, the only tractable approach is with intact protein top-down tandem mass spectrometry. Here, ultra-high-resolution FT-ICR MS and MS/MS yield quantitative relative abundances of all detected HeLa H2A and H2B isobaric and isomeric variants with a label-free...
Show moreHistone variants are known to play a central role in genome regulation and maintenance. However, many variants are inaccessible by antibody-based methods or bottom-up tandem mass spectrometry due to their highly similar sequences. For many, the only tractable approach is with intact protein top-down tandem mass spectrometry. Here, ultra-high-resolution FT-ICR MS and MS/MS yield quantitative relative abundances of all detected HeLa H2A and H2B isobaric and isomeric variants with a label-free approach. We extend the analysis to identify and relatively quantitate 16 proteoforms from 12 sequence variants of histone H2A and 10 proteoforms of histone H2B from three other cell lines: human embryonic stem cells (WA09), U937, and a prostate cancer cell line LaZ. The top-down MS/MS approach provides a path forward for more extensive elucidation of the biological role of many previously unstudied histone variants and post-translational modifications.
Show less - Date Issued
- 2016-09-02
- Identifier
- FSU_pmch_27431976, 10.1021/acs.jproteome.6b00414, PMC6261780, 27431976, 27431976
- Format
- Citation
- Title
- Quantitative assessment of fluorescent proteins.
- Creator
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Cranfill, Paula J, Sell, Brittney R, Baird, Michelle A, Allen, John R, Lavagnino, Zeno, de Gruiter, H Martijn, Kremers, Gert-Jan, Davidson, Michael W, Ustione, Alessandro,...
Show moreCranfill, Paula J, Sell, Brittney R, Baird, Michelle A, Allen, John R, Lavagnino, Zeno, de Gruiter, H Martijn, Kremers, Gert-Jan, Davidson, Michael W, Ustione, Alessandro, Piston, David W
Show less - Abstract/Description
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The advent of fluorescent proteins (FPs) for genetic labeling of molecules and cells has revolutionized fluorescence microscopy. Genetic manipulations have created a vast array of bright and stable FPs spanning blue to red spectral regions. Common to autofluorescent FPs is their tight β-barrel structure, which provides the rigidity and chemical environment needed for effectual fluorescence. Despite the common structure, each FP has unique properties. Thus, there is no single 'best' FP for...
Show moreThe advent of fluorescent proteins (FPs) for genetic labeling of molecules and cells has revolutionized fluorescence microscopy. Genetic manipulations have created a vast array of bright and stable FPs spanning blue to red spectral regions. Common to autofluorescent FPs is their tight β-barrel structure, which provides the rigidity and chemical environment needed for effectual fluorescence. Despite the common structure, each FP has unique properties. Thus, there is no single 'best' FP for every circumstance, and each FP has advantages and disadvantages. To guide decisions about which FP is right for a given application, we have quantitatively characterized the brightness, photostability, pH stability and monomeric properties of more than 40 FPs to enable straightforward and direct comparison between them. We focus on popular and/or top-performing FPs in each spectral region.
Show less - Date Issued
- 2016-07-01
- Identifier
- FSU_pmch_27240257, 10.1038/nmeth.3891, PMC4927352, 27240257, 27240257, nmeth.3891
- Format
- Citation
- Title
- Toward 20 T magnetic resonance for human brain studies: opportunities for discovery and neuroscience rationale..
- Creator
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Budinger, Thomas F, Bird, Mark D, Frydman, Lucio, Long, Joanna R, Mareci, Thomas H, Rooney, William D, Rosen, Bruce, Schenck, John F, Schepkin, Victor D, Sherry, A Dean,...
Show moreBudinger, Thomas F, Bird, Mark D, Frydman, Lucio, Long, Joanna R, Mareci, Thomas H, Rooney, William D, Rosen, Bruce, Schenck, John F, Schepkin, Victor D, Sherry, A Dean, Sodickson, Daniel K, Springer, Charles S, Thulborn, Keith R, Uğurbil, Kamil, Wald, Lawrence L
Show less - Abstract/Description
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An initiative to design and build magnetic resonance imaging (MRI) and spectroscopy (MRS) instruments at 14 T and beyond to 20 T has been underway since 2012. This initiative has been supported by 22 interested participants from the USA and Europe, of which 15 are authors of this review. Advances in high temperature superconductor materials, advances in cryocooling engineering, prospects for non-persistent mode stable magnets, and experiences gained from large-bore, high-field magnet...
Show moreAn initiative to design and build magnetic resonance imaging (MRI) and spectroscopy (MRS) instruments at 14 T and beyond to 20 T has been underway since 2012. This initiative has been supported by 22 interested participants from the USA and Europe, of which 15 are authors of this review. Advances in high temperature superconductor materials, advances in cryocooling engineering, prospects for non-persistent mode stable magnets, and experiences gained from large-bore, high-field magnet engineering for the nuclear fusion endeavors support the feasibility of a human brain MRI and MRS system with 1 ppm homogeneity over at least a 16-cm diameter volume and a bore size of 68 cm. Twelve neuroscience opportunities are presented as well as an analysis of the biophysical and physiological effects to be investigated before exposing human subjects to the high fields of 14 T and beyond.
Show less - Date Issued
- 2016-06-01
- Identifier
- FSU_pmch_27194154, 10.1007/s10334-016-0561-4, PMC5538368, 27194154, 27194154, 10.1007/s10334-016-0561-4
- Format
- Citation
- Title
- 1.1-billion-year-old Porphyrins Establish A Marine Ecosystem Dominated By Bacterial Primary Producers.
- Creator
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Gueneli, N., McKenna, A. M., Ohkouchi, N., Boreham, C. J., Beghin, J., Javaux, E. J., Brocks, J. J.
- Abstract/Description
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The average cell size of marine phytoplankton is critical for the flow of energy and nutrients from the base of the food web to higher trophic levels. Thus, the evolutionary succession of primary producers through Earth's history is important for our understanding of the radiation of modern protists similar to 800 million years ago and the emergence of eumetazoan animals similar to 200 million years later. Currently, it is difficult to establish connections between primary production and the...
Show moreThe average cell size of marine phytoplankton is critical for the flow of energy and nutrients from the base of the food web to higher trophic levels. Thus, the evolutionary succession of primary producers through Earth's history is important for our understanding of the radiation of modern protists similar to 800 million years ago and the emergence of eumetazoan animals similar to 200 million years later. Currently, it is difficult to establish connections between primary production and the proliferation of large and complex organisms because the mid-Proterozoic (similar to 1,800-800 million years ago) rock record is nearly devoid of recognizable phytoplankton fossils. We report the discovery of intact porphyrins, the molecular fossils of chlorophylls, from 1,100-million-year-old marine black shales of the Taoudeni Basin (Mauritania), 600 million years older than previous findings. The porphyrin nitrogen isotopes (delta N-15(por) = 5.6-10.2 parts per thousand) are heavier than in younger sedimentary sequences, and the isotopic offset between sedimentary bulk nitrogen and porphyrins (epsilon(por) = -5.1 to -0.5 parts per thousand) points to cyanobacteria as dominant primary producers. Based on fossil carotenoids, anoxygenic green (Chlorobiacea) and purple sulfur bacteria (Chromatiaceae) also contributed to photosynthate. The low epsilon(por) values, in combination with a lack of diagnostic eukaryotic steranes in the time interval of 1,600-1,000 million years ago, demonstrate that algae played an insignificant role in mid-Proterozoic oceans. The paucity of algae and the small cell size of bacterial phytoplankton may have curtailed the flow of energy to higher trophic levels, potentially contributing to a diminished evolutionary pace toward complex eukaryotic ecosystems and large and active organisms.
Show less - Date Issued
- 2018-07-24
- Identifier
- FSU_libsubv1_wos_000439574700004, 10.1073/pnas.1803866115
- Format
- Citation
- Title
- Persistent-current switch for pancake coils of rare earth-barium-copper-oxide high-temperature superconductor: Design and test results of a double-pancake coil operated in liquid nitrogen (77-65 K) and in solid nitrogen (60-57 K)..
- Creator
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Qu, Timing, Michael, Philip C, Voccio, John, Bascuñán, Juan, Hahn, Seungyong, Iwasa, Yukikazu
- Abstract/Description
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We present design and test results of a superconducting persistent current switch (PCS) for pancake coils of rare-earth-barium-copper-oxide, REBCO, high-temperature superconductor (HTS). Here, a REBCO double-pancake (DP) coil, 152-mm ID, 168-mm OD, 12-mm high, was wound with a no-insulation technique. We converted a ∼10-cm long section in the outermost layer of each pancake to a PCS. The DP coil was operated in liquid nitrogen (77-65 K) and in solid nitrogen (60-57 K). Over the operating...
Show moreWe present design and test results of a superconducting persistent current switch (PCS) for pancake coils of rare-earth-barium-copper-oxide, REBCO, high-temperature superconductor (HTS). Here, a REBCO double-pancake (DP) coil, 152-mm ID, 168-mm OD, 12-mm high, was wound with a no-insulation technique. We converted a ∼10-cm long section in the outermost layer of each pancake to a PCS. The DP coil was operated in liquid nitrogen (77-65 K) and in solid nitrogen (60-57 K). Over the operating temperature ranges of this experiment, the normal-state PCS enabled the DP coil to be energized; thereupon, the PCS resumed the superconducting state and the DP coil field decayed with a time constant of 100 h, which would have been nearly infinite, i.e., persistent-mode operation, were the joint across the coil terminals superconducting.
Show less - Date Issued
- 2016-08-22
- Identifier
- FSU_pmch_27647942, 10.1063/1.4961622, PMC5001974, 27647942, 27647942, 017635APL
- Format
- Citation
- Title
- A route for a strong increase of critical current in nanostrained iron-based superconductors.
- Creator
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Ozaki, Toshinori, Wu, Lijun, Zhang, Cheng, Jaroszynski, Jan, Si, Weidong, Zhou, Juan, Zhu, Yimei, Li, Qiang
- Abstract/Description
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The critical temperature T and the critical current density J determine the limits to large-scale superconductor applications. Superconductivity emerges at T. The practical current-carrying capability, measured by J, is the ability of defects in superconductors to pin the magnetic vortices, and that may reduce T. Simultaneous increase of T and J in superconductors is desirable but very difficult to realize. Here we demonstrate a route to raise both T and J together in iron-based...
Show moreThe critical temperature T and the critical current density J determine the limits to large-scale superconductor applications. Superconductivity emerges at T. The practical current-carrying capability, measured by J, is the ability of defects in superconductors to pin the magnetic vortices, and that may reduce T. Simultaneous increase of T and J in superconductors is desirable but very difficult to realize. Here we demonstrate a route to raise both T and J together in iron-based superconductors. By using low-energy proton irradiation, we create cascade defects in FeSeTe films. T is enhanced due to the nanoscale compressive strain and proximity effect, whereas J is doubled under zero field at 4.2 K through strong vortex pinning by the cascade defects and surrounding nanoscale strain. At 12 K and above 15 T, one order of magnitude of J enhancement is achieved in both parallel and perpendicular magnetic fields to the film surface.
Show less - Date Issued
- 2016-10-06
- Identifier
- FSU_pmch_27708268, 10.1038/ncomms13036, PMC5059717, 27708268, 27708268, ncomms13036
- Format
- Citation
- Title
- A flexible iron(II) complex in which zero-field splitting is resistant to structural variation.
- Creator
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Zadrozny, Joseph M., Greer, Samuel M., Hill, Stephen, Freedman, Danna E.
- Abstract/Description
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The relationship between electronic structure and zero-field splitting dictates key design parameters for magnetic molecules. In particular, to enable the directed synthesis of new electronic spin based qubits, developing complexes where zero-field splitting energies are invariant to structural changes is a critical challenge. Toward those ends, we report three salts of a new compound, a four-coordinate iron(II) complex [ Fe(C3S5)(2)](2-) ([(18-crown-6) K](+) (1), Ph4P+ (2), Bu4N+ (3)) with a...
Show moreThe relationship between electronic structure and zero-field splitting dictates key design parameters for magnetic molecules. In particular, to enable the directed synthesis of new electronic spin based qubits, developing complexes where zero-field splitting energies are invariant to structural changes is a critical challenge. Toward those ends, we report three salts of a new compound, a four-coordinate iron(II) complex [ Fe(C3S5)(2)](2-) ([(18-crown-6) K](+) (1), Ph4P+ (2), Bu4N+ (3)) with a continuous structural variation in a single parameter, the dihedral angle (theta(d)) between the two C3S52- ligands, as a function of counterion (theta(d) = 89.98(4)degrees for 1 to 72.41(2)degrees for 3). Electron paramagnetic resonance data for 1-3 reveal zero-field splitting parameters that are unusually robust to the structural variation. Mossbauer spectroscopic measurements indicate that the structural variation in theta(d) primarily affects the highest-energy 3d-orbitals (d(xz) and d(yz)) of the iron(II) ion. These orbitals have the smallest impact on the zero-field splitting parameters, thus the distortion has a minor effect on D and E. These results represent the first part of a directed effort to understand how spin state energies may be fortified against structural distortions for future applications of qubits in non-crystalline environments.
Show less - Date Issued
- 2016
- Identifier
- FSU_libsubv1_wos_000366826900047, 10.1039/c5sc02477c
- Format
- Citation
- Title
- Magnetic phase diagram of underdoped YBaCuO inferred from torque magnetization and thermal conductivity.
- Creator
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Yu, Fan, Hirschberger, Max, Loew, Toshinao, Li, Gang, Lawson, Benjamin J, Asaba, Tomoya, Kemper, J B, Liang, Tian, Porras, Juan, Boebinger, Gregory S, Singleton, John, Keimer,...
Show moreYu, Fan, Hirschberger, Max, Loew, Toshinao, Li, Gang, Lawson, Benjamin J, Asaba, Tomoya, Kemper, J B, Liang, Tian, Porras, Juan, Boebinger, Gregory S, Singleton, John, Keimer, Bernhard, Li, Lu, Ong, N Phuan
Show less - Abstract/Description
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Strong evidence for charge-density correlation in the underdoped phase of the cuprate YBaCuO was obtained by NMR and resonant X-ray scattering. The fluctuations were found to be enhanced in strong magnetic fields. Recently, 3D charge-density-wave (CDW) formation with long-range order (LRO) was observed by X-ray diffraction in [Formula: see text] 15 T. To elucidate how the CDW transition impacts the pair condensate, we have used torque magnetization to 45 T and thermal conductivity [Formula:...
Show moreStrong evidence for charge-density correlation in the underdoped phase of the cuprate YBaCuO was obtained by NMR and resonant X-ray scattering. The fluctuations were found to be enhanced in strong magnetic fields. Recently, 3D charge-density-wave (CDW) formation with long-range order (LRO) was observed by X-ray diffraction in [Formula: see text] 15 T. To elucidate how the CDW transition impacts the pair condensate, we have used torque magnetization to 45 T and thermal conductivity [Formula: see text] to construct the magnetic phase diagram in untwinned crystals with hole density = 0.11. We show that the 3D CDW transitions appear as sharp features in the susceptibility and [Formula: see text] at the fields [Formula: see text] and [Formula: see text], which define phase boundaries in agreement with spectroscopic techniques. From measurements of the melting field [Formula: see text] of the vortex solid, we obtain evidence for two vortex solid states below 8 K. At 0.5 K, the pair condensate appears to adjust to the 3D CDW by a sharp transition at 24 T between two vortex solids with very different shear moduli. At even higher (41 T), the second vortex solid melts to a vortex liquid which survives to fields well above 41 T. de Haas-van Alphen oscillations appear at fields 24-28 T, below the lower bound for the upper critical field [Formula: see text].
Show less - Date Issued
- 2016-11-08
- Identifier
- FSU_pmch_27791146, 10.1073/pnas.1612591113, PMC5111645, 27791146, 27791146, 1612591113
- Format
- Citation
- Title
- Intrinsic and extrinsic pinning in NdFeAs(O,F): vortex trapping and lock-in by the layered structure..
- Creator
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Tarantini, C, Iida, K, Hänisch, J, Kurth, F, Jaroszynski, J, Sumiya, N, Chihara, M, Hatano, T, Ikuta, H, Schmidt, S, Seidel, P, Holzapfel, B, Larbalestier, D C
- Abstract/Description
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Fe-based superconductors (FBS) present a large variety of compounds whose properties are affected to different extents by their crystal structures. Amongst them, the REFeAs(O,F) (RE1111, RE being a rare-earth element) is the family with the highest critical temperature T but also with a large anisotropy and Josephson vortices as demonstrated in the flux-flow regime in Sm1111 (T ∼ 55 K). Here we focus on the pinning properties of the lower-T Nd1111 in the flux-creep regime. We demonstrate that...
Show moreFe-based superconductors (FBS) present a large variety of compounds whose properties are affected to different extents by their crystal structures. Amongst them, the REFeAs(O,F) (RE1111, RE being a rare-earth element) is the family with the highest critical temperature T but also with a large anisotropy and Josephson vortices as demonstrated in the flux-flow regime in Sm1111 (T ∼ 55 K). Here we focus on the pinning properties of the lower-T Nd1111 in the flux-creep regime. We demonstrate that for H//c critical current density J at high temperatures is dominated by point-defect pinning centres, whereas at low temperatures surface pinning by planar defects parallel to the c-axis and vortex shearing prevail. When the field approaches the ab-planes, two different regimes are observed at low temperatures as a consequence of the transition between 3D Abrikosov and 2D Josephson vortices: one is determined by the formation of a vortex-staircase structure and one by lock-in of vortices parallel to the layers. This is the first study on FBS showing this behaviour in the full temperature, field, and angular range and demonstrating that, despite the lower T and anisotropy of Nd1111 with respect to Sm1111, this compound is substantially affected by intrinsic pinning generating a strong ab-peak in J.
Show less - Date Issued
- 2016-10-26
- Identifier
- FSU_pmch_27782196, 10.1038/srep36047, PMC5080545, 27782196, 27782196, srep36047
- Format
- Citation
- Title
- A route for a strong increase of critical current in nanostrained iron-based superconductors.
- Creator
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Ozaki, Toshinori, Wu, Lijun, Zhang, Cheng, Jaroszynski, Jan, Si, Weidong, Zhou, Juan, Zhu, Yimei, Li, Qiang
- Abstract/Description
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The critical temperature T-c and the critical current density J(c) determine the limits to large-scale superconductor applications. Superconductivity emerges at T-c. The practical current-carrying capability, measured by J(c), is the ability of defects in superconductors to pin the magnetic vortices, and that may reduce T-c. Simultaneous increase of T-c and J(c) in superconductors is desirable but very difficult to realize. Here we demonstrate a route to raise both T-c and J(c) together in...
Show moreThe critical temperature T-c and the critical current density J(c) determine the limits to large-scale superconductor applications. Superconductivity emerges at T-c. The practical current-carrying capability, measured by J(c), is the ability of defects in superconductors to pin the magnetic vortices, and that may reduce T-c. Simultaneous increase of T-c and J(c) in superconductors is desirable but very difficult to realize. Here we demonstrate a route to raise both T-c and J(c) together in iron-based superconductors. By using low-energy proton irradiation, we create cascade defects in FeSe0.5Te0.5 films. T-c is enhanced due to the nanoscale compressive strain and proximity effect, whereas J(c) is doubled under zero field at 4.2 K through strong vortex pinning by the cascade defects and surrounding nanoscale strain. At 12 K and above 15 T, one order of magnitude of J(c) enhancement is achieved in both parallel and perpendicular magnetic fields to the film surface.
Show less - Date Issued
- 2016-10-06
- Identifier
- FSU_libsubv1_wos_000385556300001, 10.1038/ncomms13036
- Format
- Citation
- Title
- Acoustic wave absorption as a probe of dynamical geometrical response of fractional quantum Hall liquids.
- Creator
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Yang, Kun
- Abstract/Description
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We show that an acoustic crystalline wave gives rise to an effect similar to that of a gravitational wave to an electron gas. Applying this idea to a two-dimensional electron gas in the fractional quantum Hall regime, this allows for experimental study of its intra-Landau level dynamical response in the long-wavelength limit. To study such response we generalize Haldane's geometrical description of fractional quantum Hall states to situations where the external metric is time dependent. We...
Show moreWe show that an acoustic crystalline wave gives rise to an effect similar to that of a gravitational wave to an electron gas. Applying this idea to a two-dimensional electron gas in the fractional quantum Hall regime, this allows for experimental study of its intra-Landau level dynamical response in the long-wavelength limit. To study such response we generalize Haldane's geometrical description of fractional quantum Hall states to situations where the external metric is time dependent. We show that such time-dependent metric (generated by acoustic wave) couples to collective modes of the system, including a quadrapolar mode at long wavelength, and magnetoroton at finite wavelength. Energies of these modes can be revealed in spectroscopic measurements, controlled by strain-induced Fermi velocity anisotropy. We argue that such geometrical probe provides a potentially highly useful alternative probe of quantum Hall liquids, in addition to the usual electromagnetic response.
Show less - Date Issued
- 2016-04-15
- Identifier
- FSU_libsubv1_wos_000374297500001, 10.1103/PhysRevB.93.161302
- Format
- Citation
- Title
- Evidence For Impact Ionization In Vanadium Dioxide.
- Creator
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Holleman, Joshua, Bishop, Michael M., Garcia, Carlos, Winfred, J. S. R. Vellore, Lee, Shinbuhm, Lee, Ho Nyung, Beekman, Christianne, Manousakis, Efstratios, McGill, Stephen A.
- Abstract/Description
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Pump-probe optical spectroscopy was used to investigate proposed charge-carrier multiplication via impact ionization in the M-1 insulating phase of VO2. By comparing the transient reflectivities of the film when pumped at less than and then more than twice the band-gap energy, we observed a larger ultrafast response with the higher energy pump color while the film was still transiently in the insulating phase. We additionally identified multiple time scales within the charge dynamics and...
Show morePump-probe optical spectroscopy was used to investigate proposed charge-carrier multiplication via impact ionization in the M-1 insulating phase of VO2. By comparing the transient reflectivities of the film when pumped at less than and then more than twice the band-gap energy, we observed a larger ultrafast response with the higher energy pump color while the film was still transiently in the insulating phase. We additionally identified multiple time scales within the charge dynamics and analyzed how these changed when the pump and probe wavelengths were varied. This experiment provided evidence that a fast carrier multiplication process, i.e., impact ionization, acts efficiently in this prototypical strongly correlated insulator, as was recently predicted by theoretical calculations.
Show less - Date Issued
- 2016-10-17
- Identifier
- FSU_libsubv1_wos_000386097100004, 10.1103/PhysRevB.94.155129
- Format
- Citation
- Title
- Evidence Of Topological Nodal-line Fermions In Zrsise And Zrsite.
- Creator
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Hu, Jin, Tang, Zhijie, Liu, Jinyu, Liu, Xue, Zhu, Yanglin, Graf, David, Myhro, Kevin, Tran, Son, Lau, Chun Ning, Wei, Jiang, Mao, Zhiqiang
- Abstract/Description
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A Dirac nodal-line semimetal phase, which represents a new quantum state of topological materials, has been experimentally realized only in a few systems, including PbTaSe2, PtSn4, and ZrSiS. In this Letter, we report evidence of nodal-line fermions in ZrSiSe and ZrSiTe probed in de Haas-van Alphen quantum oscillations. Although ZrSiSe and ZrSiTe share a similar layered structure with ZrSiS, our studies show the Fermi surface (FS) enclosing a Dirac nodal line has a 2D character in ZrSiTe, in...
Show moreA Dirac nodal-line semimetal phase, which represents a new quantum state of topological materials, has been experimentally realized only in a few systems, including PbTaSe2, PtSn4, and ZrSiS. In this Letter, we report evidence of nodal-line fermions in ZrSiSe and ZrSiTe probed in de Haas-van Alphen quantum oscillations. Although ZrSiSe and ZrSiTe share a similar layered structure with ZrSiS, our studies show the Fermi surface (FS) enclosing a Dirac nodal line has a 2D character in ZrSiTe, in contrast with 3D-like FS in ZrSiSe and ZrSiS. Another important property revealed in our experiment is that the nodal-line fermion density in this family of materials (similar to 10(20) cm(-3)) is much higher than the Dirac fermion density of other topological materials with discrete nodes. In addition, we have demonstrated ZrSiSe and ZrSiTe single crystals can be thinned down to 2D atomic thin layers through microexfoliation, which offers the first platform to explore exotic properties of topological nodal-line fermions in low dimensions.
Show less - Date Issued
- 2016-06-30
- Identifier
- FSU_libsubv1_wos_000378881300009, 10.1103/PhysRevLett.117.016602
- Format
- Citation
- Title
- Evidence From Exafs For Different Ta/ti Site Occupancy In High Critical Current Density Nb3sn Superconductor Wires.
- Creator
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Heald, Steve M., Tarantini, Chiara, Lee, Peter J., Brown, Michael D., Sung, ZuHawn, Ghosh, Arup K., Larbalestier, David C.
- Abstract/Description
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To meet critical current density, J(c), targets for the Future Circular Collider (FCC), the planned replacement for the Large Hadron Collider (LHC), the high field performance of Nb3Sn must be improved, but champion J(c) values have remained static for the last 10 years. Making the A15 phase stoichiometric and enhancing the upper critical field H-c2 by Ti or Ta dopants are the standard strategies for enhancing high field performance but detailed recent studies show that even the best modern...
Show moreTo meet critical current density, J(c), targets for the Future Circular Collider (FCC), the planned replacement for the Large Hadron Collider (LHC), the high field performance of Nb3Sn must be improved, but champion J(c) values have remained static for the last 10 years. Making the A15 phase stoichiometric and enhancing the upper critical field H-c2 by Ti or Ta dopants are the standard strategies for enhancing high field performance but detailed recent studies show that even the best modern wires have broad composition ranges. To assess whether further improvement might be possible, we employed Extended X-ray Absorption Fine Structure (EXAFS) to determine the lattice site location of dopants in modern high-performance Nb3Sn strands with J(c) values amongst the best so far achieved. Although Ti and Ta primarily occupy the Nb sites in the A15 structure, we also find significant Ta occupancy on the Sn site. These findings indicate that the best performing Ti-doped stand is strongly sub-stoichiometric in Sn and that antisite disorder likely explains its high average H-c2 behavior. These new results suggest an important role for dopant and antisite disorder in minimizing superconducting property distributions and maximizing high field J(c) properties.
Show less - Date Issued
- 2018-03-19
- Identifier
- FSU_libsubv1_wos_000427686900005, 10.1038/s41598-018-22924-3
- Format
- Citation
- Title
- Fabrication and characterization of ultraviolet photosensors from ZnO nanowires prepared using chemical bath deposition method.
- Creator
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Al-Asadi, Ahmed S., Henley, Luke Alexander, Ghosh, Sujoy, Quetz, Abdiel, Dubenko, Igor, Pradhan, Nihar, Balicas, Luis, Perera-Lopez, Nestor, Carozo, Victor, Lin, Zhong, Terrones...
Show moreAl-Asadi, Ahmed S., Henley, Luke Alexander, Ghosh, Sujoy, Quetz, Abdiel, Dubenko, Igor, Pradhan, Nihar, Balicas, Luis, Perera-Lopez, Nestor, Carozo, Victor, Lin, Zhong, Terrones, Mauricio, Talapatra, Saikat, Ali, Naushad
Show less - Abstract/Description
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Highly crystalline zinc oxide (ZnO) nanowires (NWs) were synthesized through chemical bath deposition (CBD) method by using a simple seeding technique. The process includes dispersion of commercially available ZnO nanoparticles through spraying on a desired substrate prior to the CBD growth. A typical growth period of 16 h produced ZnO NW assemblies with an average diameter of similar to 45 nm and lengths of 1-1.3 mu m, with an optical band gap of similar to 3.61 eV. The as-prepared ZnO NWs...
Show moreHighly crystalline zinc oxide (ZnO) nanowires (NWs) were synthesized through chemical bath deposition (CBD) method by using a simple seeding technique. The process includes dispersion of commercially available ZnO nanoparticles through spraying on a desired substrate prior to the CBD growth. A typical growth period of 16 h produced ZnO NW assemblies with an average diameter of similar to 45 nm and lengths of 1-1.3 mu m, with an optical band gap of similar to 3.61 eV. The as-prepared ZnO NWs were photoactive under ultra violet (UV) illumination. Photodetector devices fabricated using these NW assemblies demonstrated a high photoresponse factor of similar to 40 and 120 at room temperature under moderate UV illumination power of similar to 250 mu W/cm(2). These findings indicate the possibility of using ZnO NWs, grown using the simple method discussed in this paper, for various opto-electronic applications. (C) 2016 AIP Publishing LLC.
Show less - Date Issued
- 2016-02-28
- Identifier
- FSU_libsubv1_wos_000371601800022, 10.1063/1.4942653
- Format
- Citation
- Title
- Fractional Quantum Hall States in a Ge Quantum Well.
- Creator
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Mironov, O. A., d'Ambrumenil, N., Dobbie, A., Leadley, D. R., Suslov, A. V., Green, E.
- Abstract/Description
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Measurements of the Hall and dissipative conductivity of a strained Ge quantum well on a SiGe/(001)Si substrate in the quantum Hall regime are reported. We analyze the results in terms of thermally activated quantum tunneling of carriers from one internal edge state to another across saddle points in the long-range impurity potential. This shows that the gaps for different filling fractions closely follow the dependence predicted by theory. We also find that the estimates of the separation of...
Show moreMeasurements of the Hall and dissipative conductivity of a strained Ge quantum well on a SiGe/(001)Si substrate in the quantum Hall regime are reported. We analyze the results in terms of thermally activated quantum tunneling of carriers from one internal edge state to another across saddle points in the long-range impurity potential. This shows that the gaps for different filling fractions closely follow the dependence predicted by theory. We also find that the estimates of the separation of the edge states at the saddle are in line with the expectations of an electrostatic model in the lowest spin-polarized Landau level (LL), but not in the spin-reversed LL where the density of quasiparticle states is not high enough to accommodate the carriers required.
Show less - Date Issued
- 2016-04-27
- Identifier
- FSU_libsubv1_wos_000374964400011, 10.1103/PhysRevLett.116.176802
- Format
- Citation
- Title
- Fermi surface reconstruction in FeSe under high pressure.
- Creator
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Terashima, Taichi, Kikugawa, Naoki, Kiswandhi, Andhika, Graf, David, Choi, Eun-Sang, Brooks, James S., Kasahara, Shigeru, Watashige, Tatsuya, Matsuda, Yuji, Shibauchi, Takasada,...
Show moreTerashima, Taichi, Kikugawa, Naoki, Kiswandhi, Andhika, Graf, David, Choi, Eun-Sang, Brooks, James S., Kasahara, Shigeru, Watashige, Tatsuya, Matsuda, Yuji, Shibauchi, Takasada, Wolf, Thomas, Boehmer, Anna E., Hardy, Frederic, Meingast, Christoph, Loehneysen, Hilbert V., Uji, Shinya
Show less - Abstract/Description
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We report Shubnikov-de Haas (SdH) oscillation measurements on FeSe under high pressure up to P = 16.1 kbar. We find a sudden change in SdH oscillations at the onset of the pressure-induced antiferromagnetism at P similar to 8 kbar. We argue that this change can be attributed to a reconstruction of the Fermi surface by the antiferromagnetic order. The negative dT(c)/dP observed in a range between P similar to 8 and 12 kbar may be explained by the reduction in the density of states due to the...
Show moreWe report Shubnikov-de Haas (SdH) oscillation measurements on FeSe under high pressure up to P = 16.1 kbar. We find a sudden change in SdH oscillations at the onset of the pressure-induced antiferromagnetism at P similar to 8 kbar. We argue that this change can be attributed to a reconstruction of the Fermi surface by the antiferromagnetic order. The negative dT(c)/dP observed in a range between P similar to 8 and 12 kbar may be explained by the reduction in the density of states due to the reconstruction. The ratio of the transition temperature to the effective Fermi energy remains high under high pressure: k(B)T(c)/E-F similar to 0.1 even at P = 16.1 kbar.
Show less - Date Issued
- 2016-03-03
- Identifier
- FSU_libsubv1_wos_000371401700003, 10.1103/PhysRevB.93.094505
- Format
- Citation
- Title
- Evidence For Correlated Dynamics Near The Berezinskii-kosterlitz-thouless-like Transition In Highly Underdoped La2-xsrxcuo4.
- Creator
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Shi, Zhenzhong, Shi, Xiaoyan, Popovic, Dragana
- Abstract/Description
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A low-frequency resistance noise study in highly underdoped thick films of La2-xSrxCuO4 (x = 0.07 and 0.08) reveals slow, correlated dynamics and breaking of ergodicity near the superconducting transition of the Berezinskii-Kosterlitz-Thouless type. The observed correlated behavior is strongly suppressed by disorder.
- Date Issued
- 2016-10-05
- Identifier
- FSU_libsubv1_wos_000385239900002, 10.1103/PhysRevB.94.134503
- Format
- Citation
- Title
- Extremely Large Nonsaturating Magnetoresistance And Ultrahigh Mobility Due To Topological Surface States In The Metallic Bi2te3 Topological Insulator.
- Creator
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Shrestha, K., Chou, M., Graf, D., Yang, H. D., Lorenz, B., Chu, C. W.
- Abstract/Description
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Weak antilocalization (WAL) effects in Bi2Te3 single crystals have been investigated at high and low bulk charge-carrier concentrations. At low charge-carrier density the WAL curves scale with the normal component of the magnetic field, demonstrating the dominance of topological surface states in magnetoconductivity. At high charge-carrier density the WAL curves scale with neither the applied field nor its normal component, implying a mixture of bulk and surface conduction. WAL due to...
Show moreWeak antilocalization (WAL) effects in Bi2Te3 single crystals have been investigated at high and low bulk charge-carrier concentrations. At low charge-carrier density the WAL curves scale with the normal component of the magnetic field, demonstrating the dominance of topological surface states in magnetoconductivity. At high charge-carrier density the WAL curves scale with neither the applied field nor its normal component, implying a mixture of bulk and surface conduction. WAL due to topological surface states shows no dependence on the nature (electrons or holes) of the bulk charge carriers. The observations of an extremely large nonsaturating magnetoresistance and ultrahigh mobility in the samples with lower carrier density further support the presence of surface states. The physical parameters characterizing the WAL effects are calculated using the Hikami-LarkinNagaoka formula. At high charge-carrier concentrations, there is a greater number of conduction channels and a decrease in the phase coherence length compared to low charge-carrier concentrations. The extremely large magnetoresistance and high mobility of topological insulators have great technological value and can be exploited in magnetoelectric sensors and memory devices.
Show less - Date Issued
- 2017-05-08
- Identifier
- FSU_libsubv1_wos_000401229000004, 10.1103/PhysRevB.95.195113
- Format
- Citation
- Title
- Gate-modulated conductance of few-layer WSe2 field-effect transistors in the subgap regime.
- Creator
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Wang, Junjie, Rhodes, Daniel, Feng, Simin, Nguyen, Minh An T., Watanabe, K., Taniguchi, T., Mallouk, Thomas E., Terrones, Mauricio, Balicas, Luis, Zhu, J.
- Date Issued
- 2016-02-08
- Identifier
- FSU_libsubv1_wos_000373056300060, 10.1063/1.4941993
- Format
- Citation
- Title
- Giant Suppression Of Phononic Heat Transport In A Quantum Magnet Bicu2po6.
- Creator
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Jeon, Byung-Gu, Koteswararao, B., Park, C. B., Shu, G. J., Riggs, S. C., Moon, E. G., Chung, S. B., Chou, F. C., Kim, Kee Hoon
- Abstract/Description
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Thermal transport of quantum magnets has elucidated the nature of low energy elementary excitations and complex interplay between those excited states via strong scattering of thermal carriers. BiCu2PO6 is a unique frustrated spin-ladder compound exhibiting highly anisotropic spin excitations that contain both itinerant and localized dispersion characters along the b- and a-axes respectively. Here, we investigate thermal conductivity. of BiCu2PO6 under high magnetic fields (H) of up to 30...
Show moreThermal transport of quantum magnets has elucidated the nature of low energy elementary excitations and complex interplay between those excited states via strong scattering of thermal carriers. BiCu2PO6 is a unique frustrated spin-ladder compound exhibiting highly anisotropic spin excitations that contain both itinerant and localized dispersion characters along the b- and a-axes respectively. Here, we investigate thermal conductivity. of BiCu2PO6 under high magnetic fields (H) of up to 30 tesla. A dip-feature in., located at similar to 15 K at zero-H along all crystallographic directions, moves gradually toward lower temperature (T) with increasing H, thus resulting in giant suppression by a factor of similar to 30 near the critical magnetic field of H-c congruent to 23.5 tesla. The giant H- and T-dependent suppression of kappa can be explained by the combined result of resonant scattering of phononic heat carriers with magnetic energy levels and increased phonon scattering due to enhanced spin fluctuation at Hc, unequivocally revealing the existence of strong spin-phonon coupling. Moreover, we find an experimental indication that the remaining magnetic heat transport along the b-axis becomes almost gapless at the magnetic quantum critical point realized at H-c.
Show less - Date Issued
- 2016-11-15
- Identifier
- FSU_libsubv1_wos_000387646400002, 10.1038/srep36970
- Format
- Citation
- Title
- Geometric dependence of transport and universal behavior in three dimensional carbon nanostructures.
- Creator
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Wang, Leizhi, Yin, Ming, Jaroszynski, Jan, Park, Ju-Hyun, Mbamalu, Godwin, Datta, Timir
- Abstract/Description
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Carbon nanostructures with the spherical voids exhibit interesting temperature and magnetic field dependent transport properties. By increasing the void size, the structures are tuned from metallic to insulating; in addition, the magnetoresistance (MR) is enhanced. Our investigation in the magnetic fields (B) up to 18 T at temperatures (T) from 250 mK to 20K shows that at high temperatures (T>2 K), the MR crosses over from quadratic to a non-saturating linear dependence with increasing...
Show moreCarbon nanostructures with the spherical voids exhibit interesting temperature and magnetic field dependent transport properties. By increasing the void size, the structures are tuned from metallic to insulating; in addition, the magnetoresistance (MR) is enhanced. Our investigation in the magnetic fields (B) up to 18 T at temperatures (T) from 250 mK to 20K shows that at high temperatures (T>2 K), the MR crosses over from quadratic to a non-saturating linear dependence with increasing magnetic field. Furthermore, all MR data in this temperature regime collapse onto a single curve as a universal function of B/T, following Kohler's rule. Remarkably, the MR also exhibits orientation insensitivity, i.e., it displays a response independent of the direction on the magnetic field. Published by AIP Publishing.
Show less - Date Issued
- 2016-09-19
- Identifier
- FSU_libsubv1_wos_000384558700054, 10.1063/1.4963261
- Format
- Citation
- Title
- Fate Of Spinons At The Mott Point.
- Creator
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Lee, Tsung-Han, Florens, Serge, Dobrosavljevic, Vladimir
- Abstract/Description
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Gapless spin liquids have recently been observed in several frustrated Mott insulators, with elementary spin excitations-"spinons"-reminiscent of degenerate Fermi systems. However, their precise role at the Mott point, where charge fluctuations begin to proliferate, remains controversial and ill understood. Here we present the simplest theoretical framework that treats the dynamics of emergent spin and charge excitations on the same footing, providing a new physical picture of the Mott metal...
Show moreGapless spin liquids have recently been observed in several frustrated Mott insulators, with elementary spin excitations-"spinons"-reminiscent of degenerate Fermi systems. However, their precise role at the Mott point, where charge fluctuations begin to proliferate, remains controversial and ill understood. Here we present the simplest theoretical framework that treats the dynamics of emergent spin and charge excitations on the same footing, providing a new physical picture of the Mott metal-to-insulator transition at half filing. We identify a generic orthogonality mechanism leading to strong damping of spinons, arising as soon as the Mott gap closes. Our results indicate that spinons should not play a significant role within the high-temperature quantum critical regime above the Mott point-in striking agreement with all available experiments.
Show less - Date Issued
- 2016-09-20
- Identifier
- FSU_libsubv1_wos_000383849400011, 10.1103/PhysRevLett.117.136601
- Format
- Citation
- Title
- Frustrated Magnetism In The Tetragonal Cose Analog Of Superconducting Fese.
- Creator
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Wilfong, Brandon, Zhou, Xiuquan, Vivanco, Hector, Campbell, Daniel J., Wang, Kefeng, Graf, Dave, Paglione, Johnpierre, Rodriguez, Efrain
- Abstract/Description
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Recently synthesized metastable tetragonal CoSe, isostructural to the FeSe superconductor, offers a new avenue for investigating systems in close proximity to the iron-based superconductors. We present magnetic and transport property measurements on powders and single crystals of CoSe. High field magnetic susceptibility measurements indicate a suppression of the previously reported 10 K ferromagnetic transition with the magnetic susceptibility, exhibiting time dependence below the proposed...
Show moreRecently synthesized metastable tetragonal CoSe, isostructural to the FeSe superconductor, offers a new avenue for investigating systems in close proximity to the iron-based superconductors. We present magnetic and transport property measurements on powders and single crystals of CoSe. High field magnetic susceptibility measurements indicate a suppression of the previously reported 10 K ferromagnetic transition with the magnetic susceptibility, exhibiting time dependence below the proposed transition. Dynamic scaling analysis of the time dependence yields a critical relaxation time of tau* = 0.064 +/- 0.008 s which in turn yields activation energy E-a(*) = 14.84 +/- 0.59 K and an ideal glass temperature T-0(*) = 8.91 +/- 0.09 K from Vogel-Fulcher analysis. No transition is observed in resistivity and specific heat measurements, but both measurements indicate that CoSe is metallic. These results are interpreted on the basis of CoSe exhibiting frustrated magnetic ordering arising from competing magnetic interactions. Arrott analysis of single crystal magnetic susceptibility has indicated the transition temperature occurs in close proximity to previous reports and that the magnetic moment lies solely in the ab plane. The results have implications for understanding the relationship between magnetism and transport properties in the iron chalcogenide superconductors.
Show less - Date Issued
- 2018-03-08
- Identifier
- FSU_libsubv1_wos_000426901700002, 10.1103/PhysRevB.97.104408
- Format
- Citation
- Title
- Gutzwiller renormalization group.
- Creator
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Lanata, Nicola, Yao, Yong-Xin, Deng, Xiaoyu, Wang, Cai-Zhuang, Ho, Kai-Ming, Kotliar, Gabriel
- Abstract/Description
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We develop a variational scheme called the "Gutzwiller renormalization group" (GRG), which enables us to calculate the ground state of Anderson impurity models (AIM) with arbitrary numerical precision. Our method exploits the low-entanglement property of the ground state of local Hamiltonians in combination with the framework of the Gutzwiller wave function and indicates that the ground state of the AIM has a very simple structure, which can be represented very accurately in terms of a...
Show moreWe develop a variational scheme called the "Gutzwiller renormalization group" (GRG), which enables us to calculate the ground state of Anderson impurity models (AIM) with arbitrary numerical precision. Our method exploits the low-entanglement property of the ground state of local Hamiltonians in combination with the framework of the Gutzwiller wave function and indicates that the ground state of the AIM has a very simple structure, which can be represented very accurately in terms of a surprisingly small number of variational parameters. We perform benchmark calculations of the single-band AIM that validate our theory and suggest that the GRG might enable us to study complex systems beyond the reach of the other methods presently available and pave the way to interesting generalizations, e.g., to nonequilibrium transport in nanostructures.
Show less - Date Issued
- 2016-01-06
- Identifier
- FSU_libsubv1_wos_000367665400002, 10.1103/PhysRevB.93.045103
- Format
- Citation
- Title
- H-1-h-2 Cross-polarization Nmr In Fast Spinning Solids By Adiabatic Sweeps.
- Creator
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Wi, Sungsool, Schurko, Robert, Frydman, Lucio
- Abstract/Description
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Cross-polarization (CP) experiments employing frequency-swept radiofrequency (rf) pulses have been successfully used in static spin systems for obtaining broadband signal enhancements. These experiments have been recently extended to heteronuclear I, S = spin-1/2 nuclides under magic-angle spinning (MAS), by applying adiabatic inversion pulses along the S (low-gamma) channel while simultaneously applying a conventional spin-locking pulse on the I-channel (H-1). This study explores an...
Show moreCross-polarization (CP) experiments employing frequency-swept radiofrequency (rf) pulses have been successfully used in static spin systems for obtaining broadband signal enhancements. These experiments have been recently extended to heteronuclear I, S = spin-1/2 nuclides under magic-angle spinning (MAS), by applying adiabatic inversion pulses along the S (low-gamma) channel while simultaneously applying a conventional spin-locking pulse on the I-channel (H-1). This study explores an extension of this adiabatic frequency sweep concept to quadrupolar nuclei, focusing on CP from H-1 (I = 1/2) to H-2 spins (S = 1) undergoing fast MAS (nu(r) = 60 kHz). A number of new features emerge, including zero- and double-quantum polarization transfer phenomena that depend on the frequency offsets of the swept pulses, the rf pulse powers, and the MAS spinning rate. An additional mechanism found operational in the H-1-H-2 CP case that was absent in the spin-1/2 counterpart, concerns the onset of a pseudo-static zero- quantum CP mode, driven by a quadrupole-modulated rf/dipolar recoupling term arising under the action of MAS. The best CP conditions found at these fast spinning rates correspond to double-quantum transfers, involving weak H-2 rf field strengths. At these easily attainable (ca. 10 kHz) rf field conditions, adiabatic level-crossings among the {vertical bar 1 ,vertical bar 0 ,broken vertical bar-1} m(S) energy levels, which are known to complicate the CP MAS of quadrupolar nuclei, are avoided. Moreover, the CP line shapes generated in this manner are very close to the ideal H-2 MAS spectral line shapes, facilitating the extraction of quadrupolar coupling parameters. All these features were corroborated with experiments on model compounds and justified using numerical simulations and average Hamiltonian theory models. Potential applications of these new phenomena, as well as extensions to higher spins S, are briefly discussed.
Show less - Date Issued
- 2017-03-14
- Identifier
- FSU_libsubv1_wos_000397313300011, 10.1063/1.4976980
- Format
- Citation
- Title
- Magnetotransport in double quantum well with inverted energy spectrum: HgTe/CdHgTe.
- Creator
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Yakunin, M. V., Suslov, A. V., Popov, M. R., Novik, E. G., Dvoretsky, S. A., Mikhailov, N. N.
- Abstract/Description
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We present an experimental study of the double-quantum-well (DQW) system made of two-dimensional layers with inverted energy band spectrum: HgTe. The magnetotransport reveals a considerably larger overlap of the conduction and valence subbands than in known HgTe single quantum wells (QW), which may be regulated here by an applied gate voltage V-g. This large overlap manifests itself in a much higher critical field B-c separating the range above it with a plain behavior of the Hall...
Show moreWe present an experimental study of the double-quantum-well (DQW) system made of two-dimensional layers with inverted energy band spectrum: HgTe. The magnetotransport reveals a considerably larger overlap of the conduction and valence subbands than in known HgTe single quantum wells (QW), which may be regulated here by an applied gate voltage V-g. This large overlap manifests itself in a much higher critical field B-c separating the range above it with a plain behavior of the Hall magnetoresistance rho(xy) (B), where the quantum peculiarities shift linearly with V-g, and the range below with a complicated behavior. In the latter case, specific structures in rho(xy) (B) are formed like a double-N-shaped rho(xy) (B), reentrant sign-alternating quantum Hall effect with transitions into a zero-filling-factor state, etc., which are clearly manifested here due to better magnetic quantization at high fields, as compared to the features seen earlier in a single HgTe QW. The coexisting electrons and holes were found in the whole investigated range of positive and negative V-g as revealed (i) from fits to the low-field N-shaped rho(xy) (B), (ii) from the Fourier analysis of oscillations in rho(xx) (B), and (iii) from a specific behavior of rho(xy) (B) at high positive V-g. A peculiar feature here is that the found electron density n remains almost constant in the whole range of investigated V-g while the hole density p drops down from the value a factor of 6 larger than n at extreme negative V-g to almost zero at extreme positive V-g passing through the charge-neutrality point. We show that this difference between n and p stems from an order of magnitude larger density of states for holes in the lateral valence subband maxima than for electrons in the conduction subband minimum. We analyze our observations on the basis of a calculated picture of magnetic levels in a DQW and suggest that their specificity is due to (i) a nonmonotonic course of the valence subband magnetic levels and an oscillating behavior of the valence subband top versus field due to lateral maxima in the energy spectrum, (ii) a reduced gap between the lowest-electron and the highest-hole magnetic levels where the electron- and hole-type localized states are superposed, and (iii) a possible formation of the interlayer electron-hole excitons.
Show less - Date Issued
- 2016-02-12
- Identifier
- FSU_libsubv1_wos_000370025100005, 10.1103/PhysRevB.93.085308
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- Citation
- Title
- Magnetoinfrared spectroscopic study of thin Bi2Te3 single crystals.
- Creator
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Tung, L.-C., Yu, W., Cadden-Zimansky, P., Miotkowski, I., Chen, Y. P., Smirnov, D., Jiang, Z.
- Abstract/Description
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Thin Bi2Te3 single crystals laid on Scotch tape are investigated by Fourier transform infrared spectroscopy at 4 K and in a magnetic field up to 35 T. The magnetotransmittance spectra of the Bi2Te3/tape composite are analyzed as a stacked-slab system, and the average thickness of Bi2Te3 is estimated to be 6.4 +/- 1.7 mu m. The optical conductivity of Bi2Te3 at different magnetic fields is then extracted, and we find that the magnetic field modifies the optical conductivity in the following...
Show moreThin Bi2Te3 single crystals laid on Scotch tape are investigated by Fourier transform infrared spectroscopy at 4 K and in a magnetic field up to 35 T. The magnetotransmittance spectra of the Bi2Te3/tape composite are analyzed as a stacked-slab system, and the average thickness of Bi2Te3 is estimated to be 6.4 +/- 1.7 mu m. The optical conductivity of Bi2Te3 at different magnetic fields is then extracted, and we find that the magnetic field modifies the optical conductivity in the following ways: (1) Field-induced transfer of the optical weight from the lower-frequency regime (< 250 cm(-1)) to the higher-frequency regime (> 250 cm(-1)) due to the redistribution of charge carriers across the Fermi surface. (2) Evolving of a Fano-resonance-like spectral feature from an antiresonance to a resonance with increasing magnetic field. Such behavior can be attributed to the electron-phonon interactions between the E-u(1) optical phonon mode and the continuum of electronic transitions. (3) Cyclotron resonance resulting from the intervalence band Landau level transitions, which can be described by the electrodynamics of massive Dirac holes.
Show less - Date Issued
- 2016-02-29
- Identifier
- FSU_libsubv1_wos_000371398500002, 10.1103/PhysRevB.93.085140
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- Citation
- Title
- Magnetoelectric Coupling Through The Spin Flop Transition In Ni3teo6.
- Creator
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Yokosuk, M. O., al-Wahish, Amal, Artyukhin, Sergey, O'Neal, K. R., Mazumdar, D., Chen, P., Yang, Junjie, Oh, Yoon Seok, McGill, Stephen A., Haule, K., Cheong, Sang-Wook,...
Show moreYokosuk, M. O., al-Wahish, Amal, Artyukhin, Sergey, O'Neal, K. R., Mazumdar, D., Chen, P., Yang, Junjie, Oh, Yoon Seok, McGill, Stephen A., Haule, K., Cheong, Sang-Wook, Vanderbilt, David, Musfeldt, J. L.
Show less - Abstract/Description
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We combined high field optical spectroscopy and first principles calculations to analyze the electronic structure of Ni3TeO6 across the 53 K and 9 T magnetic transitions, both of which are accompanied by large changes in electric polarization. The color properties are sensitive to magnetic order due to field-induced changes in the crystal field environment, with those around Ni1 and Ni2 most affected. These findings advance the understanding of magnetoelectric coupling in materials in which...
Show moreWe combined high field optical spectroscopy and first principles calculations to analyze the electronic structure of Ni3TeO6 across the 53 K and 9 T magnetic transitions, both of which are accompanied by large changes in electric polarization. The color properties are sensitive to magnetic order due to field-induced changes in the crystal field environment, with those around Ni1 and Ni2 most affected. These findings advance the understanding of magnetoelectric coupling in materials in which magnetic 3d centers coexist with nonmagnetic heavy chalcogenide cations.
Show less - Date Issued
- 2016-09-30
- Identifier
- FSU_libsubv1_wos_000385971800013, 10.1103/PhysRevLett.117.147402
- Format
- Citation
- Title
- Measurement of Long-Range Near-Side Two-Particle Angular Correlations in pp Collisions at root s=13 TeV.
- Creator
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Khachatryan, V., Sirunyan, A. M., Tumasyan, A., Adam, W., Asilar, E., Bergauer, T., Brandstetter, J., Brondolin, E., Dragicevic, M., Ero, J., Flechl, M., Friedl, M., Fruhwirth,...
Show moreKhachatryan, V., Sirunyan, A. M., Tumasyan, A., Adam, W., Asilar, E., Bergauer, T., Brandstetter, J., Brondolin, E., Dragicevic, M., Ero, J., Flechl, M., Friedl, M., Fruhwirth, R., Ghete, V. M., Hartl, C., Hormann, N., Hrubec, J., Jeitler, M., Knunz, V., Konig, A., Krammer, M., Kratschmer, I., Liko, D., Matsushita, T., Mikulec, I., Rabady, D., Rahbaran, B., Rohringer, H., Schieck, J., Schofbeck, R., Strauss, J., Treberer-Treberspurg, W., Waltenberger, W., Wulz, C.-E., Mossolov, V., Shumeiko, N., Gonzalez, J. Suarez, Alderweireldt, S., Cornelis, T., De Wolf, E. A., Janssen, X., Knutsson, A., Lauwers, J., Luyckx, S., Van de Klundert, M., Van Haevermaet, H., Van Mechelen, P., Van Remortel, N., Van Spilbeeck, A., Abu Zeid, S., Blekman, F., D'Hondt, J., Daci, N., De Bruyn, I., Deroover, K., Heracleous, N., Keaveney, J., Lowette, S., Moreels, L., Olbrechts, A., Python, Q., Strom, D., Tavernier, S., Van Doninck, W., Van Mulders, P., Van Onsem, G. P., Van Parijs, I., Barria, P., Brun, H., Caillol, C., Clerbaux, B., De Lentdecker, G., Fasanella, G., Favart, L., Grebenyuk, A., Karapostoli, G., Lenzi, T., Leonard, A., Maerschalk, T., Marinov, A., Pernie, L., Randle-conde, A., Seva, T., Vander Velde, C., Vanlaer, P., Yonamine, R., Zenoni, F., Zhang, F., Beernaert, K., Benucci, L., Cimmino, A., Crucy, S., Dobur, D., Fagot, A., Garcia, G., Gul, M., Mccartin, J., Rios, A. A. Ocampo, Poyraz, D., Ryckbosch, D., Salva, S., Sigamani, M., Tytgat, M., Van Driessche, W., Yazgan, E., Zaganidis, N., Basegmez, S., Beluffi, C., Bondu, O., Brochet, S., Bruno, G., Caudron, A., Ceard, L., Da Silveira, G. G., Delaere, C., Favart, D., Forthomme, L., Giammanco, A., Hollar, J., Jafari, A., Jez, P., Komm, M., Lemaitre, V., Mertens, A., Musich, M., Nuttens, C., Perrini, L., Pin, A., Piotrzkowski, K., Popov, A., Quertenmont, L., Selvaggi, M., Marono, M. Vidal, Beliy, N., Hammad, G. H., Alda Junior, W. L., Alves, F. L., Alves, G. A., Brito, L., Correa Martins Junior, M., Hamer, M., Hensel, C., Moraes, A., Pol, M. E., Rebello Teles, P., Belchior Batista Das Chagas, E., Carvalho, W., Chinellato, J., Custodio, A., Da Costa, E. M., De Jesus Damiao, D., De Oliveira Martins, C., Fonseca De Souza, S., Huertas Guativa, L. M., Malbouisson, H., Matos Figueiredo, D., Mora Herrera, C., Mundim, L., Nogima, H., Prado Da Silva, W. L., Santoro, A., Sznajder, A., Tonelli Manganote, E. J., Vilela Pereira, A., Ahuja, S., Bernardes, C. A., De Souza Santos, A., Dogra, S., Fernandez Perez Tomei, T. R., Gregores, E. M., Mercadante, P. G., Moon, C. S., Novaes, S. F., Padula, Sandra S., Romero Abad, D., Ruiz Vargas, J. C., Aleksandrov, A., Hadjiiska, R., Iaydjiev, P., Rodozov, M., Stoykova, S., Sultanov, G., Vutova, M., Dimitrov, A., Glushkov, I., Litov, L., Pavlov, B., Petkov, P., Ahmad, M., Bian, J. G., Chen, G. M., Chen, H. S., Chen, M., Cheng, T., Du, R., Jiang, C. H., Plestina, R., Romeo, F., Shaheen, S. M., Spiezia, A., Tao, J., Wang, C., Wang, Z., Zhang, H., Asawatangtrakuldee, C., Ban, Y., Li, Q., Liu, S., Mao, Y., Qian, S. J., Wang, D., Xu, Z., Avila, C., Cabrera, A., Sierra, L. F. Chaparro, Florez, C., Gomez, J. P., Gomez Moreno, B., Sanabria, J. C., Godinovic, N., Lelas, D., Puljak, I., Cipriano, P. M. Ribeiro, Antunovic, Z., Kovac, M., Brigljevic, V., Kadija, K., Luetic, J., Micanovic, S., Sudic, L., Attikis, A., Mavromanolakis, G., Mousa, J., Nicolaou, C., Ptochos, F., Razis, P. A., Rykaczewski, H., Bodlak, M., Finger, M., Finger, M., El-khateeb, E., Elkafrawy, T., Mohamed, A., Salama, E., Calpas, B., Kadastik, M., Murumaa, M., Raidal, M., Tiko, A., Veelken, C., Eerola, P., Pekkanen, J., Voutilainen, M., Harkonen, J., Karimaki, V., Kinnunen, R., Lampen, T., Lassila-Perini, K., Lehti, S., Linden, T., Luukka, P., Peltola, T., Tuominen, E., Tuominiemi, J., Tuovinen, E., Wendland, L., Talvitie, J., Tuuva, T., Besancon, M., Couderc, F., Dejardin, M., Denegri, D., Fabbro, B., Faure, J. L., Favaro, C., Ferri, F., Ganjour, S., Givernaud, A., Gras, P., de Monchenault, G. Hamel, Jarry, P., Locci, E., Machet, M., Malcles, J., Rander, J., Rosowsky, A., Titov, M., Zghiche, A., Antropov, I., Baffioni, S., Beaudette, F., Busson, P., Cadamuro, L., Chapon, E., Charlot, C., Davignon, O., Filipovic, N., de Cassagnac, R. Granier, Jo, M., Lisniak, S., Mastrolorenzo, L., Mine, P., Naranjo, I. N., Nguyen, M., Ochando, C., Ortona, G., Paganini, P., Pigard, P., Regnard, S., Salerno, R., Sauvan, J. B., Sirois, Y., Strebler, T., Yilmaz, Y., Zabi, A., Agram, J.-L., Andrea, J., Aubin, A., Bloch, D., Brom, J.-M., Buttignol, M., Chabert, E. C., Chanon, N., Collard, C., Conte, E., Coubez, X., Fontaine, J.-C., Gele, D., Goerlach, U., Goetzmann, C., Le Bihan, A.-C., Merlin, J. A., Skovpen, K., Van Hove, P., Gadrat, S., Beauceron, S., Bernet, C., Boudoul, G., Bouvier, E., Montoya, C. A. Carrillo, Chierici, R., Contardo, D., Courbon, B., Depasse, P., El Mamouni, H., Fan, J., Fay, J., Gascon, S., Gouzevitch, M., Ille, B., Lagarde, F., Laktineh, I. B., Lethuillier, M., Mirabito, L., Pequegnot, A. L., Perries, S., Alvarez, J. D. Ruiz, Sabes, D., Sgandurra, L., Sordini, V., Vander Donckt, M., Verdier, P., Viret, S., Toriashvili, T., Tsamalaidze, Z., Autermann, C., Beranek, S., Feld, L., Heister, A., Kiesel, M. K., Klein, K., Lipinski, M., Ostapchuk, A., Preuten, M., Raupach, F., Schael, S., Schulte, J. F., Verlage, T., Weber, H., Zhukov, V., Ata, M., Brodski, M., Dietz-Laursonn, E., Duchardt, D., Endres, M., Erdmann, M., Erdweg, S., Esch, T., Fischer, R., Guth, A., Hebbeker, T., Heidemann, C., Hoepfner, K., Knutzen, S., Kreuzer, P., Merschmeyer, M., Meyer, A., Millet, P., Mukherjee, S., Olschewski, M., Padeken, K., Papacz, P., Pook, T., Radziej, M., Reithler, H., Rieger, M., Scheuch, F., Sonnenschein, L., Teyssier, D., Thueer, S., Cherepanov, V., Erdogan, Y., Fluegge, G., Geenen, H., Geisler, M., Hoehle, F., Kargoll, B., Kress, T., Kuessel, Y., Kuensken, A., Lingemann, J., Nehrkorn, A., Nowack, A., Nugent, I. M., Pistone, C., Pooth, O., Stahl, A., Martin, M. Aldaya, Asin, I., Bartosik, N., Behnke, O., Behrens, U., Bell, A. J., Borras, K., Burgmeier, A., Campbell, A., Costanza, F., Pardos, C. Diez, Dolinska, G., Dooling, S., Dorland, T., Eckerlin, G., Eckstein, D., Eichhorn, T., Flucke, G., Gallo, E., Garcia, J. Garay, Geiser, A., Gizhko, A., Gunnellini, P., Hauk, J., Hempel, M., Jung, H., Kalogeropoulos, A., Karacheban, O., Kasemann, M., Katsas, P., Kieseler, J., Kleinwort, C., Korol, I., Lange, W., Leonard, J., Lipka, K., Lobanov, A., Lohmann, W., Mankel, R., Marfin, I., Melzer-Pellmann, I.-A., Meyer, A. B., Mittag, G., Mnich, J., Mussgiller, A., Naumann-Emme, S., Nayak, A., Ntomari, E., Perrey, H., Pitzl, D., Placakyte, R., Raspereza, A., Roland, B., Sahin, M. O., Saxena, P., Schoerner-Sadenius, T., Seitz, C., Spannagel, S., Trippkewitz, K. D., Walsh, R., Wissing, C., Blobel, V., Vignali, M. Centis, Draeger, A. R., Erfle, J., Garutti, E., Goebel, K., Gonzalez, D., Goerner, M., Haller, J., Hoffmann, M., Hoeing, R. S., Junkes, A., Klanner, R., Kogler, R., Kovalchuk, N., Lapsien, T., Lenz, T., Marchesini, I., Marconi, D., Meyer, M., Nowatschin, D., Ott, J., Pantaleo, F., Peiffer, T., Perieanu, A., Pietsch, N., Poehlsen, J., Rathjens, D., Sander, C., Scharf, C., Schettler, H., Schleper, P., Schlieckau, E., Schmidt, A., Schwandt, J., Sola, V., Stadie, H., Steinbrueck, G., Tholen, H., Troendle, D., Usai, E., Vanelderen, L., Vanhoefer, A., Vormwald, B., Barth, C., Baur, S., Baus, C., Berger, J., Boeser, C., Butz, E., Chwalek, T., Colombo, F., De Boer, W., Descroix, A., Dierlamm, A., Fink, S., Frensch, F., Friese, R., Giffels, M., Gilbert, A., Haitz, D., Hartmann, F., Heindl, S. M., Husemann, U., Katkov, I., Kornmayer, A., Pardo, P. Lobelle, Maier, B., Mildner, H., Mozer, M. U., Mueller, T., Mueller, Th, Plagge, M., Quast, G., Rabbertz, K., Roecker, S., Roscher, F., Schroeder, M., Sieber, G., Simonis, H. J., Stober, F. M., Ulrich, R., Wagner-Kuhr, J., Wayand, S., Weber, M., Weiler, T., Williamson, S., Woehrmann, C., Wolf, R., Anagnostou, G., Daskalakis, G., Geralis, T., Giakoumopoulou, V. A., Kyriakis, A., Loukas, D., Psallidas, A., Topsis-Giotis, I., Agapitos, A., Kesisoglou, S., Panagiotou, A., Saoulidou, N., Tziaferi, E., Evangelou, I., Flouris, G., Foudas, C., Kokkas, P., Loukas, N., Manthos, N., Papadopoulos, I., Paradas, E., Strologas, J., Bencze, G., Hajdu, C., Hazi, A., Hidas, P., Horvath, D., Sikler, F., Veszpremi, V., Vesztergombi, G., Zsigmond, A. J., Beni, N., Czellar, S., Karancsi, J., Molnar, J., Szillasi, Z., Bartok, M., Makovec, A., Raics, P., Trocsanyi, Z. L., Ujvari, B., Choudhury, S., Mal, P., Mandal, K., Sahoo, D. K., Sahoo, N., Swain, S. K., Bansal, S., Beri, S. B., Bhatnagar, V., Chawla, R., Gupta, R., Bhawandeep, U., Kalsi, A. K., Kaur, A., Kaur, M., Kumar, R., Mehta, A., Mittal, M., Singh, J. B., Walia, G., Kumar, Ashok, Bhardwaj, A., Choudhary, B. C., Garg, R. B., Malhotra, S., Naimuddin, M., Nishu, N., Ranjan, K., Sharma, R., Sharma, V., Bhattacharya, S., Chatterjee, K., Dey, S., Dutta, S., Jain, Sa, Majumdar, N., Modak, A., Mondal, K., Mukhopadhyay, S., Roy, A., Roy, D., Chowdhury, S. Roy, Sarkar, S., Sharan, M., Abdulsalam, A., Chudasama, R., Dutta, D., Jha, V., Kumar, V., Mohanty, A. K., Pant, L. M., Shukla, P., Topkar, A., Aziz, T., Banerjee, S., Bhowmik, S., Chatterjee, R. M., Dewanjee, R. K., Dugad, S., Ganguly, S., Ghosh, S., Guchait, M., Gurtu, A., Kole, G., Kumar, S., Mahakud, B., Maity, M., Majumder, G., Mazumdar, K., Mitra, S., Mohanty, G. B., Parida, B., Sarkar, T., Sur, N., Sutar, B., Wickramage, N., Chauhan, S., Dube, S., Kapoor, A., Kothekar, K., Sharma, S., Bakhshiansohi, H., Behnamian, H., Etesami, S. M., Fahim, A., Goldouzian, R., Khakzad, M., Najafabadi, M. Mohammadi, Naseri, M., Mehdiabadi, S. Paktinat, Hosseinabadi, F. Rezaei, Safarzadeh, B., Zeinali, M., Felcini, M., Grunewald, M., Abbrescia, M., Calabria, C., Caputo, C., Colaleo, A., Creanza, D., Cristella, L., De Filippis, N., De Palma, M., Fiore, L., Iaselli, G., Maggi, G., Maggi, M., Miniello, G., My, S., Nuzzo, S., Pompili, A., Pugliese, G., Radogna, R., Ranieri, A., Selvaggi, G., Silvestris, L., Venditti, R., Abbiendi, G., Battilana, C., Benvenuti, A. C., Bonacorsi, D., Braibant-Giacomelli, S., Brigliadori, L., Campanini, R., Capiluppi, P., Castro, A., Cavallo, F. R., Chhibra, S. S., Codispoti, G., Cuffiani, M., Dallavalle, G. M., Fabbri, F., Fanfani, A., Fasanella, D., Giacomelli, P., Grandi, C., Guiducci, L., Marcellini, S., Masetti, G., Montanari, A., Navarria, F. L., Perrotta, A., Rossi, A. M., Rovelli, T., Siroli, G. P., Tosi, N., Travaglini, R., Cappello, G., Chiorboli, M., Costa, S., Di Mattia, A., Giordano, F., Potenza, R., Tricomi, A., Tuve, C., Barbagli, G., Ciulli, V., Civinini, C., D'Alessandro, R., Focardi, E., Gori, V., Lenzi, P., Meschini, M., Paoletti, S., Sguazzoni, G., Viliani, L., Benussi, L., Bianco, S., Fabbri, F., Piccolo, D., Primavera, F., Calvelli, V., Ferro, F., Lo Vetere, M., Monge, M. R., Robutti, E., Tosi, S., Brianza, L., Dinardo, M. E., Fiorendi, S., Gennai, S., Gerosa, R., Ghezzi, A., Govoni, P., Malvezzi, S., Manzoni, R. A., Marzocchi, B., Menasce, D., Moroni, L., Paganoni, M., Pedrini, D., Ragazzi, S., Redaelli, N., de Fatis, T. Tabarelli, Buontempo, S., Cavallo, N., Di Guida, S., Esposito, M., Fabozzi, F., Iorio, A. O. M., Lanza, G., Lista, L., Meola, S., Merola, M., Paolucci, P., Sciacca, C., Thyssen, F., Azzi, P., Bacchetta, N., Benato, L., Bisello, D., Boletti, A., Branca, A., Carlin, R., Checchia, P., Dall'Osso, M., Dorigo, T., Dosselli, U., Gasparini, F., Gasparini, U., Gonella, F., Gozzelino, A., Kanishchev, K., Lacaprara, S., Margoni, M., Meneguzzo, A. T., Pazzini, J., Pozzobon, N., Ronchese, P., Simonetto, F., Torassa, E., Tosi, M., Zanetti, M., Zotto, P., Zucchetta, A., Zumerle, G., Braghieri, A., Magnani, A., Montagna, P., Ratti, S. P., Re, V., Riccardi, C., Salvini, P., Vai, I., Vitulo, P., Solestizi, L. Alunni, Bilei, G. M., Ciangottini, D., Fano, L., Lariccia, P., Mantovani, G., Menichelli, M., Saha, A., Santocchia, A., Androsov, K., Azzurri, P., Bagliesi, G., Bernardini, J., Boccali, T., Castaldi, R., Ciocci, M. A., Dell'Orso, R., Donato, S., Fedi, G., Foa, L., Giassi, A., Grippo, M. T., Ligabue, F., Lomtadze, T., Martini, L., Messineo, A., Palla, F., Rizzi, A., Savoy-Navarro, A., Serban, A. T., Spagnolo, P., Tenchini, R., Tonelli, G., Venturi, A., Verdini, P. G., Barone, L., Cavallari, F., D'imperio, G., Del Re, D., Diemoz, M., Gelli, S., Jorda, C., Longo, E., Margaroli, F., Meridiani, P., Organtini, G., Paramatti, R., Preiato, F., Rahatlou, S., Rovelli, C., Santanastasio, F., Traczyk, P., Amapane, N., Arcidiacono, R., Argiro, S., Arneodo, M., Bellan, R., Biino, C., Cartiglia, N., Costa, M., Covarelli, R., Degano, A., Demaria, N., Finco, L., Kiani, B., Mariotti, C., Maselli, S., Migliore, E., Monaco, V., Monteil, E., Obertino, M. M., Pacher, L., Pastrone, N., Pelliccioni, M., Angioni, G. L. Pinna, Ravera, F., Romero, A., Ruspa, M., Sacchi, R., Solano, A., Staiano, A., Belforte, S., Candelise, V., Casarsa, M., Cossutti, F., Della Ricca, G., Gobbo, B., La Licata, C., Marone, M., Schizzi, A., Zanetti, A., Kropivnitskaya, A., Nam, S. K., Kim, D. H., Kim, G. 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Show less - Abstract/Description
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Results on two-particle angular correlations for charged particles produced in pp collisions at a center-of- mass energy of 13 TeV are presented. The data were taken with the CMS detector at the LHC and correspond to an integrated luminosity of about 270 nb(-1). The correlations are studied over a broad range of pseudorapidity (vertical bar eta vertical bar 2.0), near-side (Delta phi approximate to 0) structure emerges in the two-particle Delta eta-Delta phi correlation functions. The...
Show moreResults on two-particle angular correlations for charged particles produced in pp collisions at a center-of- mass energy of 13 TeV are presented. The data were taken with the CMS detector at the LHC and correspond to an integrated luminosity of about 270 nb(-1). The correlations are studied over a broad range of pseudorapidity (vertical bar eta vertical bar < 2.4) and over the full azimuth (phi) as a function of charged particle multiplicity and transverse momentum (p(T)). In high-multiplicity events, a long-range (vertical bar Delta eta vertical bar > 2.0), near-side (Delta phi approximate to 0) structure emerges in the two-particle Delta eta-Delta phi correlation functions. The magnitude of the correlation exhibits a pronounced maximum in the range 1.0 < p(T) < 2.0 GeV/c and an approximately linear increase with the charged particle multiplicity, with an overall correlation strength similar to that found in earlier pp data at root s = 7 TeV. The present measurement extends the study of near-side long-range correlations up to charged particle multiplicities N-ch similar to 180, a region so far unexplored in pp collisions. The observed longrange correlations are compared to those seen in pp, pPb, and PbPb collisions at lower collision energies.
Show less - Date Issued
- 2016-04-27
- Identifier
- FSU_libsubv1_wos_000374964400005, 10.1103/PhysRevLett.116.172302
- Format
- Citation
- Title
- Measurement Of Spin Correlations In Tf Production Using The Matrix Element Method In The Muon Plus Jets Final State In Pp Collisions At Root S=8 Tev.
- Creator
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Khachatryan, V., Sirunyan, A. M., Tumasyan, A., Adam, W., Asilar, E., Bergauer, T., Brandstetter, J., Brondolin, E., Dragicevic, M., Eroe, J., Flechl, M., Friedl, M., Fruehwirth...
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Show less - Abstract/Description
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The consistency of the spin correlation strength in top quark pair production with the standard model (SM) prediction is tested in the muon+jets final state. The events are selected from pp collisions, collected by the CMS detector, at a centre-of-mass energy of 8 TeV, corresponding to an integrated luminosity of 19.7 fb(-1). The data are compared with the expectation for the spin correlation predicted by the SM and with the expectation of no correlation. Using a template fit method, the...
Show moreThe consistency of the spin correlation strength in top quark pair production with the standard model (SM) prediction is tested in the muon+jets final state. The events are selected from pp collisions, collected by the CMS detector, at a centre-of-mass energy of 8 TeV, corresponding to an integrated luminosity of 19.7 fb(-1). The data are compared with the expectation for the spin correlation predicted by the SM and with the expectation of no correlation. Using a template fit method, the fraction of events that show SM spin correlations is measured to be 0.72 0.08 (stat)(-013)(+015) (syst), representing the most precise measurement of this quantity in the muon+jets final state to date. (C) 2016 The Author. Published by Elsevier B.V. This is an open access article under the CC BY license (http://creativecommons.orglicenses/by/4.01).
Show less - Date Issued
- 2016-07-10
- Identifier
- FSU_libsubv1_wos_000377330500045, 10.1016/j.physletb.2016.05.005
- Format
- Citation
- Title
- Measurement Of The Cp-violating Weak Phase Phi(s) And The Decay Width Difference Delta Gamma(s) Using The B-s(0) -> J/psi Phi (1020) Decay Channel In Pp Collisions At Root S=8 Tev.
- Creator
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Khachatryan, V., Sirunyan, A. M., Tumasyan, A., Adam, W., Asilar, E., Bergauer, T., Brandstetter, J., Brondolin, E., Dragicevic, M., Eroe, J., Flechl, M., Friedl, M., Fruehwirth...
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Show less - Abstract/Description
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The CP-violating weak phase phi(s) of the B-s(0) meson and the decay width difference Delta Gamma(s) of the B-s(0) light and heavy mass eigenstates are measured with the CMS detector at the LHC using a data sample of B-s(0)-> J/psi phi(1020) -> mu(+)mu-K+K- decays. The analysed data set corresponds to an integrated luminosity of 19.7 fb(-1) collected in pp collisions at a centre-of-mass energy of 8 TeV. A total of 49200 reconstructed B-s(0) decays are used to extract the values of phi(s) and...
Show moreThe CP-violating weak phase phi(s) of the B-s(0) meson and the decay width difference Delta Gamma(s) of the B-s(0) light and heavy mass eigenstates are measured with the CMS detector at the LHC using a data sample of B-s(0)-> J/psi phi(1020) -> mu(+)mu-K+K- decays. The analysed data set corresponds to an integrated luminosity of 19.7 fb(-1) collected in pp collisions at a centre-of-mass energy of 8 TeV. A total of 49200 reconstructed B-s(0) decays are used to extract the values of phi(s) and Delta Gamma(s) by performing a time dependent and flavour-tagged angular analysis of the mu(+)mu-K+K- final state. The weak phase is measured to be phi(s) =-0.075 +/- 0.097 (stat) +/- 0.031 (syst) rad, and the decay width difference is Delta Gamma(s) = 0.095 +/- 0.013 (stat) +/- 0.007 (syst) ps(-1). (C) 2016 CERN for the benefit of the CMS Collaboration. Published by Elsevier B.V. This is an open access article under the CC BY license (http://creativecommons.org/licenses/by/4.0/). Funded by SCOAP(3).
Show less - Date Issued
- 2016-06-10
- Identifier
- FSU_libsubv1_wos_000376800300014, 10.1016/j.physletb.2016.03.046
- Format
- Citation
- Title
- Large Fermi Surface of Heavy Electrons at the Border of Mott Insulating State in NiS2.
- Creator
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Friedemann, S., Chang, H., Gamza, M. B., Reiss, P., Chen, X., Alireza, P., Coniglio, W. A., Graf, D., Tozer, S., Grosche, F. M.
- Abstract/Description
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One early triumph of quantum physics is the explanation why some materials are metallic whereas others are insulating. While a treatment based on single electron states is correct for most materials this approach can fail spectacularly, when the electrostatic repulsion between electrons causes strong correlations. Not only can these favor new and subtle forms of matter, such as magnetism or superconductivity, they can even cause the electrons in a half-filled energy band to lock into position...
Show moreOne early triumph of quantum physics is the explanation why some materials are metallic whereas others are insulating. While a treatment based on single electron states is correct for most materials this approach can fail spectacularly, when the electrostatic repulsion between electrons causes strong correlations. Not only can these favor new and subtle forms of matter, such as magnetism or superconductivity, they can even cause the electrons in a half-filled energy band to lock into position, producing a correlated, or Mott insulator. The transition into the Mott insulating state raises important fundamental questions. Foremost among these is the fate of the electronic Fermi surface and the associated charge carrier mass, as the Mott transition is approached. We report the first direct observation of the Fermi surface on the metallic side of a Mott insulating transition by high pressure quantum oscillatory measurements in NiS2. Our results point at a large Fermi surface consistent with Luttinger's theorem and a strongly enhanced quasiparticle effective mass. These two findings are in line with central tenets of the Brinkman-Rice picture of the correlated metal near the Mott insulating state and rule out alternative scenarios in which the carrier concentration vanishes continuously at the metal-insulator transition.
Show less - Date Issued
- 2016-05-12
- Identifier
- FSU_libsubv1_wos_000375656900001, 10.1038/srep25335
- Format
- Citation
- Title
- Magnetochromic Sensing And Size-dependent Collective Excitations In Iron Oxide Nanoparticles.
- Creator
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O'Neal, Kenneth R., Patete, Jonathan M., Chen, Peng, Nanavati, Ruhani, Holinsworth, Brian S., Smith, Jacqueline M., Marques, Carlos, Simonson, Jack W., Aronson, Meigan C.,...
Show moreO'Neal, Kenneth R., Patete, Jonathan M., Chen, Peng, Nanavati, Ruhani, Holinsworth, Brian S., Smith, Jacqueline M., Marques, Carlos, Simonson, Jack W., Aronson, Meigan C., McGill, Stephen A., Wong, Stanislaus S., Musfeldt, Janice L.
Show less - Abstract/Description
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We combine optical and magneto-optical spectroscopies with complementary vibrational and magnetic property measurements to reveal finite length scale effects in nanoscale alpha-Fe2O3. Analysis of the d-to-d on-site excitations uncovers enhanced color contrast at particle sizes below approximately 75 nm due to size-induced changes in spin-charge coupling that are suppressed again below the superparamagnetic limit. These findings provide a general strategy for amplifying magnetochromism in...
Show moreWe combine optical and magneto-optical spectroscopies with complementary vibrational and magnetic property measurements to reveal finite length scale effects in nanoscale alpha-Fe2O3. Analysis of the d-to-d on-site excitations uncovers enhanced color contrast at particle sizes below approximately 75 nm due to size-induced changes in spin-charge coupling that are suppressed again below the superparamagnetic limit. These findings provide a general strategy for amplifying magnetochromism in alpha-Fe2O3 and other iron-containing nanomaterials that may be useful for advanced sensing applications. We also unravel the size dependence of collective excitations in this iconic antiferromagnet.
Show less - Date Issued
- 2017-03-10
- Identifier
- FSU_libsubv1_wos_000396013400006, 10.1103/PhysRevB.95.125416
- Format
- Citation
- Title
- Magnetic Torque Anomaly In The Quantum Limit Of Weyl Semimetals.
- Creator
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Moll, Philip J. W., Potter, Andrew C., Nair, Nityan L., Ramshaw, B. J., Modic, K. A., Riggs, Scott, Zeng, Bin, Ghimire, Nirmal J., Bauer, Eric D., Kealhofer, Robert, Ronning,...
Show moreMoll, Philip J. W., Potter, Andrew C., Nair, Nityan L., Ramshaw, B. J., Modic, K. A., Riggs, Scott, Zeng, Bin, Ghimire, Nirmal J., Bauer, Eric D., Kealhofer, Robert, Ronning, Filip, Analytis, James G.
Show less - Abstract/Description
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Electrons in materials with linear dispersion behave as massless Weyl-or Dirac-quasi-particles, and continue to intrigue due to their close resemblance to elusive ultra-relativistic particles as well as their potential for future electronics. Yet the experimental signatures of Weyl-fermions are often subtle and indirect, in particular if they coexist with conventional, massive quasiparticles. Here we show a pronounced anomaly in the magnetic torque of the Weyl semimetal NbAs upon entering the...
Show moreElectrons in materials with linear dispersion behave as massless Weyl-or Dirac-quasi-particles, and continue to intrigue due to their close resemblance to elusive ultra-relativistic particles as well as their potential for future electronics. Yet the experimental signatures of Weyl-fermions are often subtle and indirect, in particular if they coexist with conventional, massive quasiparticles. Here we show a pronounced anomaly in the magnetic torque of the Weyl semimetal NbAs upon entering the quantum limit state in high magnetic fields. The torque changes sign in the quantum limit, signalling a reversal of the magnetic anisotropy that can be directly attributed to the topological nature of the Weyl electrons. Our results establish that anomalous quantum limit torque measurements provide a direct experimental method to identify and distinguish Weyl and Dirac systems.
Show less - Date Issued
- 2016-08
- Identifier
- FSU_libsubv1_wos_000381905000001, 10.1038/ncomms12492
- Format
- Citation
- Title
- Magnetic Phases Of The Quasi-two-dimensional Antiferromagnet Cucro2 On A Triangular Lattice.
- Creator
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Sakhratov, Yu A., Svistov, L. E., Kuhns, P. L., Zhou, H. D., Reyes, A. P.
- Abstract/Description
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We have carried out Cu-63,Cu-65 NMR spectra measurements in a magnetic field up to about 45 T on a single crystal of a multiferroic triangular antiferromagnet CuCrO2. The measurements were performed for magnetic fields aligned along the crystal c axis. Field and temperature evolution of the spectral shape demonstrates a number of phase transitions. It was found that the 3D magnetic ordering takes place in the low field range (H less than or similar to 15 T). At higher fields magnetic...
Show moreWe have carried out Cu-63,Cu-65 NMR spectra measurements in a magnetic field up to about 45 T on a single crystal of a multiferroic triangular antiferromagnet CuCrO2. The measurements were performed for magnetic fields aligned along the crystal c axis. Field and temperature evolution of the spectral shape demonstrates a number of phase transitions. It was found that the 3D magnetic ordering takes place in the low field range (H less than or similar to 15 T). At higher fields magnetic structures form within individual triangular planes whereas the spin directions of the magnetic ions from neighboring planes are not correlated. It is established that the 2D-3D transition is hysteretic in field and temperature. Line-shape analysis reveals several possible magnetic structures existing within individual planes for different phases of CuCrO2. Within certain regions on the magnetic H-T phase diagram of CuCrO2 a 3D magnetic ordering with tensor order parameter is expected.
Show less - Date Issued
- 2016-09-12
- Identifier
- FSU_libsubv1_wos_000383138700003, 10.1103/PhysRevB.94.094410
- Format
- Citation
- Title
- Magnetic Ground States of the Rare-Earth Tripod Kagome Lattice Mg2RE3Sb3O14 (RE = Gd,Dy,Er).
- Creator
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Dun, Z. L., Trinh, J., Li, K., Lee, M., Chen, K. W., Baumbach, R., Hu, Y. F., Wang, Y. X., Choi, E. S., Shastry, B. S., Ramirez, A. P., Zhou, H. D.
- Abstract/Description
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We present the structural and magnetic properties of a new compound family, Mg2RE3Sb3O14 (RE = Gd, Dy, Er), with a hitherto unstudied frustrating lattice, the "tripod kagome" structure. Susceptibility (ac, dc) and specific heat exhibit features that are understood within a simple Luttinger-Tisza-type theory. For RE = Gd, we found long-ranged order (LRO) at 1.65 K, which is consistent with a 120 degrees structure, demonstrating the importance of diople interactions for this 2D Heisenberg...
Show moreWe present the structural and magnetic properties of a new compound family, Mg2RE3Sb3O14 (RE = Gd, Dy, Er), with a hitherto unstudied frustrating lattice, the "tripod kagome" structure. Susceptibility (ac, dc) and specific heat exhibit features that are understood within a simple Luttinger-Tisza-type theory. For RE = Gd, we found long-ranged order (LRO) at 1.65 K, which is consistent with a 120 degrees structure, demonstrating the importance of diople interactions for this 2D Heisenberg system. For RE = Dy, LRO at 0.37 K is related to the "kagome spin ice" physics for a 2D system. This result shows that the tripod kagome structure accelerates the transition to LRO predicted for the related pyrochlore systems. For RE = Er, two transitions, at 80 mK and 2.1 K are observed, suggesting the importance of quantum fluctuations for this putative XY system.
Show less - Date Issued
- 2016-04-12
- Identifier
- FSU_libsubv1_wos_000373773600014, 10.1103/PhysRevLett.116.157201
- Format
- Citation
- Title
- Magnetic-field-induced changes in superparamagnetic cluster dynamics in the martensitic phase of Ni43Co7Mn40Sn10.
- Creator
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Kuhns, P. L., Hoch, M. J. R., Yuan, S., Reyes, A. P., Srivastava, V., James, R. D., Leighton, C.
- Abstract/Description
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The off-stoichiometric Heusler alloys, such as Ni50Mn25+yX25-y (X = Sn, In, Ga, etc.), have been extensively investigated using a variety of experimental techniques to probe their interesting and potentially useful magnetic properties. Recent Mn-55 nuclear magnetic resonance (NMR) experiments, carried out largely in zero field (ZF) and making use of the large internal hyperfine field at the nuclear sites, have demonstrated the power of this approach in determining the ground state magnetic...
Show moreThe off-stoichiometric Heusler alloys, such as Ni50Mn25+yX25-y (X = Sn, In, Ga, etc.), have been extensively investigated using a variety of experimental techniques to probe their interesting and potentially useful magnetic properties. Recent Mn-55 nuclear magnetic resonance (NMR) experiments, carried out largely in zero field (ZF) and making use of the large internal hyperfine field at the nuclear sites, have demonstrated the power of this approach in determining the ground state magnetic characteristics of these materials. In particular, the results reveal that distinct nanoscale ferromagnetic and antiferromagnetic phases coexist. A key parameter used in interpreting the NMR data is the transverse relaxation time T-2 which, inter alia, determines the NMR blocking temperature T-B(NMR) of magnetic regions. The present experiments on a polycrystalline sample of a specific illustrative alloy, Ni43Co7Mn40Sn10, which has received considerable attention, show that the application of relatively small external fields, comparable to or greater than the local anisotropy field in the ferromagnetic cluster regions, produces dramatic changes in T-2 and hence T-B(NMR). The experimental findings are discussed using an extended version of a recently proposed nanocluster model for superparamagnetic systems. It is demonstrated that the field and temperature induced changes in T-2 provide a significant test of the model and lead to a notable advance in applying the NMR technique to the investigation of the magnetic properties of this type of alloy. Published by AIP Publishing.
Show less - Date Issued
- 2016-06-20
- Identifier
- FSU_libsubv1_wos_000379039900023, 10.1063/1.4954732
- Format
- Citation
- Title
- Magnetic properties of doped Mn-Ga alloys made by mechanical milling and heat treatment.
- Creator
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Brown, Daniel R., Han, Ke, Siegrist, Theo, Besara, Tiglet, Niu, Rongmei
- Abstract/Description
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Mn-Ga alloys have shown hard magnetic properties, even though these alloys contain no rare-earth metals. However, much work is needed before rare-earth magnets can be replaced. We have examined the magnetic properties of bulk alloys made with partial replacement of both the Mn and Ga elements in the Mn0.8Ga0.2 system. Bulk samples of Mn-Ga-Bi, Mn-Ga-Al, Mn-Fe-Ga and Mn-(FeB)-Ga alloys were fabricated and studied using mechanically milling and heat treatments while altering the atomic...
Show moreMn-Ga alloys have shown hard magnetic properties, even though these alloys contain no rare-earth metals. However, much work is needed before rare-earth magnets can be replaced. We have examined the magnetic properties of bulk alloys made with partial replacement of both the Mn and Ga elements in the Mn0.8Ga0.2 system. Bulk samples of Mn-Ga-Bi, Mn-Ga-Al, Mn-Fe-Ga and Mn-(FeB)-Ga alloys were fabricated and studied using mechanically milling and heat treatments while altering the atomic percentage of the third element between 2.5 and 20 at%. The ternary alloy exhibits all hard magnetic properties at room temperature with large coercivity. Annealed Mn-Ga-X bulk composites exhibit high coercivities up to 16.6 kOe and remanence up to 9.8 emu/g, that is increased by 115% over the binary system. (C) 2016 Author(s).
Show less - Date Issued
- 2016-05
- Identifier
- FSU_libsubv1_wos_000377962500181, 10.1063/1.4943931
- Format
- Citation
- Title
- Magnetic Ground States And Magnetodielectric Effect In Rcr(bo3)(2) (r = Y And Ho).
- Creator
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Sinclair, R., Zhou, H. D., Lee, M., Choi, S., Li, G., Hong, T., Calder, S.
- Abstract/Description
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The layered perovskites RCr(BO3)(2) (R = Y and Ho) with magnetic triangular lattices were studied by performing ac/dc susceptibility, specific heat, elastic and inelastic neutron scattering, and dielectric constant measurements. The results show (i) both samples' Cr3+ spins order in a canted antiferromagnetic structure with TN around 8-9 K, while the Ho3+ ions do not order down to T = 1.5 K in HoCr(BO3)(2); (ii) when a critical magnetic field HC around 2-3 T is applied below TN, the Cr3+...
Show moreThe layered perovskites RCr(BO3)(2) (R = Y and Ho) with magnetic triangular lattices were studied by performing ac/dc susceptibility, specific heat, elastic and inelastic neutron scattering, and dielectric constant measurements. The results show (i) both samples' Cr3+ spins order in a canted antiferromagnetic structure with TN around 8-9 K, while the Ho3+ ions do not order down to T = 1.5 K in HoCr(BO3)(2); (ii) when a critical magnetic field HC around 2-3 T is applied below TN, the Cr3+ spins in the Y compound and both the Cr3+ and Ho3+ spins in the Ho compound order in a ferromagnetic state; (iii) both samples exhibit dielectric constant anomalies around the transition temperature and critical field, but the Ho compound displays a much stronger magnetodielectric response. We speculate that this is due to the magnetostriction, which depends on both the Cr3+ and the Ho3+ ions' ordering in the Ho compound. Moreover, by using linear spin-wave theory to simulate the inelastic neutron scattering data, we estimated the Y compound's intralayer and interlayer exchange strengths as ferromagnetic J(1) = -0.12 meV and antiferromagnetic J(2) = 0.014 meV, respectively. The competition between different kinds of superexchange interactions results in the ferromagnetic intralayer interaction.
Show less - Date Issued
- 2017-05-08
- Identifier
- FSU_libsubv1_wos_000401223700002, 10.1103/PhysRevB.95.174410
- Format
- Citation
- Title
- Magnetic Field Tuning Of An Excitonic Insulator Between The Weak And Strong Coupling Regimes In Quantum Limit Graphite.
- Creator
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Zhu, Z., McDonald, R. D., Shekhter, A., Ramshaw, B. J., Modic, K. A., Balakirev, F. F., Harrison, N.
- Abstract/Description
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The excitonic insulator phase has long been predicted to form in proximity to a band gap opening in the underlying band structure. The character of the pairing is conjectured to crossover from weak (BCS-like) to strong coupling (BEC-like) as the underlying band structure is tuned from the metallic to the insulating side of the gap opening. Here we report the high-magnetic field phase diagram of graphite to exhibit just such a crossover. By way of comprehensive angle-resolved magnetoresistance...
Show moreThe excitonic insulator phase has long been predicted to form in proximity to a band gap opening in the underlying band structure. The character of the pairing is conjectured to crossover from weak (BCS-like) to strong coupling (BEC-like) as the underlying band structure is tuned from the metallic to the insulating side of the gap opening. Here we report the high-magnetic field phase diagram of graphite to exhibit just such a crossover. By way of comprehensive angle-resolved magnetoresistance measurements, we demonstrate that the underlying band gap opening occurs inside the magnetic field-induced phase, paving the way for a systematic study of the BCS-BEC-like crossover by means of conventional condensed matter probes.
Show less - Date Issued
- 2017-05-04
- Identifier
- FSU_libsubv1_wos_000408480400001, 10.1038/s41598-017-01693-5
- Format
- Citation
- Title
- Measurement of the t(t)over-bar production cross section in the all-jets final state in pp collisions at root s=8TeV.
- Creator
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Khachatryan, V., Sirunyan, A. M., Tumasyan, A., Adam, W., Asilar, E., Bergauer, T., Brandstetter, J., Brondolin, E., Dragicevic, M., Eroe, J., Flechl, M., Friedl, M., Fruehwirth...
Show moreKhachatryan, V., Sirunyan, A. M., Tumasyan, A., Adam, W., Asilar, E., Bergauer, T., Brandstetter, J., Brondolin, E., Dragicevic, M., Eroe, J., Flechl, M., Friedl, M., Fruehwirth, R., Ghete, M., Hartl, C., Hoerrmann, N., Hrubec, J., Jeitler, M., Knuenz, V., Koenig, A., Krammer, M., Kraetschmer, I., Liko, D., Matsushita, T., Mikulec, I., Rabady, D., Rahbaran, B., Rohringer, H., Schieck, J., Schoefbeck, R., Strauss, J., Treberer-Treberspurg, W., Waltenberger, W., Wulz, C.-E., Mossolov, V., Shumeiko, N., Gonzalez, J. Suarez, Alderweireldt, S., Cornelis, T., De Wolf, E. A., Janssen, X., Knutsson, A., Lauwers, J., Luyckx, S., Van de Klundert, M., Van Haevermaet, H., Van Mechelen, P., Van Remortel, N., Van Spilbeeck, A., Abu Zeid, S., Blekman, F., D'Hondt, J., Daci, N., De Bruyn, I., Deroover, K., Heracleous, N., Keaveney, J., Lowette, S., Moreels, L., Olbrechts, A., Python, Q., Strom, D., Tavernier, S., Van Doninck, W., Van Mulders, P., Van Onsem, G. P., Van Parijs, I., Barria, P., Brun, H., Caillol, C., Clerbaux, B., De Lentdecker, G., Fasanella, G., Favart, L., Grebenyuk, A., Karapostoli, G., Lenzi, T., Leonard, A., Maerschalk, T., Marinov, A., Pernie, L., Randle-conde, A., Reis, T., Seva, T., Vander Velde, C., Vanlaer, P., Yonamine, R., Zenoni, F., Zhang, F., Beernaert, K., Benucci, L., Cimmino, A., Crucy, S., Dobur, D., Fagot, A., Garcia, G., Gul, M., Mccartin, J., Rios, A. A. Ocampo, Poyraz, D., Ryckbosch, D., Salva, S., Sigamani, M., Strobbe, N., Tytgat, M., Van Driessche, W., Yazgan, E., Zaganidis, N., Basegmez, S., Beluffi, C., Bondu, O., Brochet, S., Bruno, G., Caudron, A., Ceard, L., Da Silveira, G. G., Delaere, C., Favart, D., Forthomme, L., Giammanco, A., Hollar, J., Jafari, A., Jez, P., Komm, M., Lemaitre, V., Mertens, A., Nuttens, C., Perrini, L., Pin, A., Piotrzkowski, K., Popov, A., Quertenmont, L., Selvaggi, M., Marono, M. Vidal, Beliy, N., Hammad, G. H., Alda Junior, W. L., Alves, F. L., Alves, G. A., Brito, L., Martins Junior, M. Correa, Hamer, M., Hensel, C., Herrera, C. Mora, Moraes, A., Pol, M. E., Teles, P. Rebello, Batista Das Chagas, E. Belchior, Carvalho, W., Chinellato, J., Custodio, A., Da Costa, E. M., Damiao, D. De Jesus, Martins, C. De Oliveira, De Souza, S. Fonseca, Huertas Guativa, L. M., Malbouisson, H., Figueiredo, D. Matos, Mundim, L., Nogima, H., Prado Da Silva, W. L., Santoro, A., Sznajder, A., Tonelli Manganote, E. J., Pereira, A. Vilela, Ahuja, S., Bernardes, C. A., Santos, A. De Souza, Dogra, S., Fernandez Perez Tomei, T. R., Gregores, E. M., Mercadante, P. G., Moon, C. S., Novaes, S. F., Padula, Sandra S., Abad, D. Romero, Ruiz Vargas, J. C., Aleksandrov, A., Hadjiiska, R., Iaydjiev, P., Rodozov, M., Stoykova, S., Sultanov, G., Vutova, M., Dimitrov, A., Glushkov, I., Litov, L., Pavlov, B., Petkov, P., Ahmad, M., Bian, J. G., Chen, G. M., Chen, H. S., Chen, M., Cheng, T., Du, R., Jiang, C. H., Plestina, R., Romeo, F., Shaheen, S. M., Tao, J., Wang, C., Wang, Z., Zhang, H., Asawatangtrakuldee, C., Ban, Y., Li, Q., Liu, S., Mao, Y., Qian, S. J., Wang, D., Xu, Z., Avila, C., Cabrera, A., Chaparro Sierra, L. F., Florez, C., Gomez, J. P., Gomez Moreno, B., Sanabria, J. C., Godinovic, N., Lelas, D., Puljak, I., Cipriano, P. M. Ribeiro, Antunovic, Z., Kovac, M., Brigljevic, V., Kadija, K., Luetic, J., Micanovic, S., Sudic, L., Attikis, A., Mavromanolakis, G., Mousa, J., Nicolaou, C., Ptochos, F., Razis, P. A., Rykaczewski, H., Bodlak, M., Finger, M., Finger, M., Abdelalim, A. A., Awad, A., El Sawy, M., Mahrous, A., Radi, A., Calpas, B., Kadastik, M., Murumaa, M., Raidal, M., Tiko, A., Veelken, C., Eerola, P., Pekkanen, J., Voutilainen, M., Harkonen, J., Karimaki, V., Kinnunen, R., Lampen, T., Lassila-Perini, K., Lehti, S., Linden, T., Luukka, P., Maenpaa, T., Peltola, T., Tuominen, E., Tuominiemi, J., Tuovinen, E., Wendland, L., Talvitie, J., Tuuva, T., Besancon, M., Couderc, F., Dejardin, M., Denegri, D., Fabbro, B., Faure, J. L., Favaro, C., Ferri, F., Ganjour, S., Givernaud, A., Gras, P., de Monchenault, G. Hamel, Jarry, P., Locci, E., Machet, M., Malcles, J., Rander, J., Rosowsky, A., Titov, M., Zghiche, A., Antropov, I., Baffioni, S., Beaudette, F., Busson, P., Cadamuro, L., Chapon, E., Charlot, C., Dahms, T., Davignon, O., Filipovic, N., Florent, A., de Cassagnac, R. Granier, Lisniak, S., Mastrolorenzo, L., Mine, P., Naranjo, I. N., Nguyen, M., Ochando, C., Ortona, G., Paganini, P., Pigard, P., Regnard, S., Salerno, R., Sauvan, J. B., Sirois, Y., Strebler, T., Yilmaz, Y., Zabi, A., Agram, J.-L., Andrea, J., Aubin, A., Bloch, D., Brom, J.-M., Buttignol, M., Chabert, E. C., Chanon, N., Collard, C., Conte, E., Coubez, X., Fontaine, J.-C., Gele, D., Goerlach, U., Goetzmann, C., Le Bihan, A.-C., Merlin, J. A., Skovpen, K., Van Hove, P., Gadrat, S., Beauceron, S., Bernet, C., Boudoul, G., Bouvier, E., Montoya, C. A. Carrillo, Chierici, R., Contardo, D., Courbon, B., Depasse, P., El Mamouni, H., Fan, J., Fay, J., Gascon, S., Gouzevitch, M., Ille, B., Lagarde, F., Laktineh, I. B., Lethuillier, M., Mirabito, L., Pequegnot, A. L., Perries, S., Alvarez, J. D. Ruiz, Sabes, D., Sgandurra, L., Sordini, V., Vander Donckt, M., Verdier, P., Viret, S., Toriashvili, T., Tsamalaidze, Z., Autermann, C., Beranek, S., Edelhoff, M., Feld, L., Heister, A., Kiesel, M. K., Klein, K., Lipinski, M., Ostapchuk, A., Preuten, M., Raupach, F., Schael, S., Schulte, J. F., Verlage, T., Weber, H., Wittmer, B., Zhukov, V., Ata, M., Brodski, M., Dietz-Laursonn, E., Duchardt, D., Endres, M., Erdmann, M., Erdweg, S., Esch, T., Fischer, R., Gueth, A., Hebbeker, T., Heidemann, C., Hoepfner, K., Klingebiel, D., Knutzen, S., Kreuzer, P., Merschmeyer, M., Meyer, A., Millet, P., Olschewski, M., Padeken, K., Papacz, P., Pook, T., Radziej, M., Reithler, H., Rieger, M., Scheuch, F., Sonnenschein, L., Teyssier, D., Thueer, S., Cherepanov, V., Erdogan, Y., Flugge, G., Geenen, H., Geisler, M., Hoehle, F., Kargoll, B., Kress, T., Kuessel, Y., Kunsken, A., Lingemann, J., Nehrkorn, A., Nowack, A., Nugent, I. M., Pistone, C., Pooth, O., Stahl, A., Martin, M. Aldaya, Asin, I., Bartosik, N., Behnke, O., Behrens, U., Bell, A. J., Borras, K., Burgmeier, A., Cakir, A., Calligaris, L., Campbell, A., Choudhury, S., Costanza, F., Pardos, C. Diez, Dolinska, G., Dooling, S., Dorland, T., Eckerlin, G., Eckstein, D., Eichhorn, T., Flucke, G., Gallo, E., Garcia, J. Garay, Geiser, A., Gizhko, A., Gunnellini, P., Hauk, J., Hempel, M., Jung, H., Kalogeropoulos, A., Karacheban, O., Kasemann, M., Katsas, P., Kieseler, J., Kleinwort, C., Korol, I., Lange, W., Leonard, J., Lipka, K., Lobanov, A., Lohmann, W., Mankel, R., Marfin, I., Melzer-Pellmann, I.-A., Meyer, A. B., Mittag, G., Mnich, J., Mussgiller, A., Naumann-Emme, S., Nayak, A., Ntomari, E., Perrey, H., Pitzl, D., Placakyte, R., Raspereza, A., Roland, B., Sahin, M. Oe, Saxena, P., Schoerner-Sadenius, T., Schroeder, M., Seitz, C., Spannagel, S., Trippkewitz, K. D., Walsh, R., Wissing, C., Blobel, V., Vignali, M. Centis, Draeger, A. R., Erfle, J., Garutti, E., Goebel, K., Gonzalez, D., Goerner, M., Haller, J., Hoffmann, M., Hoeng, R. S., Junkes, A., Klanner, R., Kogler, R., Lapsien, T., Lenz, T., Marchesini, I., Marconi, D., Meyer, M., Nowatschin, D., Ott, J., Pantaleo, F., Peiffer, T., Perieanu, A., Pietsch, N., Poehlsen, J., Rathjens, D., Sander, C., Schettler, H., Schleper, P., Schlieckau, E., Schmidt, A., Schwandt, J., Seidel, M., Sola, V., Stadie, H., Steinbruck, G., Tholen, H., Troendle, D., Usai, E., Vanelderen, L., Vanhoefer, A., Vormwald, B., Akbiyik, M., Barth, C., Baus, C., Berger, J., Boeser, C., Butz, E., Chwalek, T., Colombo, F., De Boer, W., Descroix, A., Dierlamm, A., Fink, S., Frensch, F., Giffels, M., Gilbert, A., Hartmann, F., Heindl, S. M., Husemann, U., Katkov, I., Kornmayer, A., Pardo, P. Lobelle, Maier, B., Mildner, H., Mozer, M. U., Mueller, T., Mueller, Th, Plagge, M., Quast, G., Rabbertz, K., Roecker, S., Roscher, F., Simonis, H. J., Stober, F. M., Ulrich, R., Wagner-Kuhr, J., Wayand, S., Weber, M., Weiler, T., Woehrmann, C., Wolf, R., Anagnostou, G., Daskalakis, G., Geralis, T., Giakoumopoulou, V. A., Kyriakis, A., Loukas, D., Psallidas, A., Topsis-Giotis, I., Agapitos, A., Kesisoglou, S., Panagiotou, A., Saoulidou, N., Tziaferi, E., Evangelou, I., Flouris, G., Foudas, C., Kokkas, P., Loukas, N., Manthos, N., Papadopoulos, I., Paradas, E., Strologas, J., Bencze, G., Hajdu, C., Hazi, A., Hidas, P., Horvath, D., Sikler, F., Veszpremi, V., Vesztergombi, G., Zsigmond, A. J., Beni, N., Czellar, S., Karancsi, J., Molnar, J., Szillasi, Z., Bartok, M., Makovec, A., Raics, P., Trocsanyi, Z. L., Ujvari, B., Mal, P., Mandal, K., Sahoo, D. K., Sahoo, N., Swain, S. K., Bansal, S., Beri, S. B., Bhatnagar, V., Chawla, R., Gupta, R., Bhawandeep, U., Kalsi, A. K., Kaur, A., Kaur, M., Kumar, R., Mehta, A., Mittal, M., Singh, J. B., Walia, G., Kumar, Ashok, Bhardwaj, A., Choudhary, B. C., Garg, R. 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Show less - Abstract/Description
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The cross section for tt production in the all-jets final state is measured in pp collisions at a centre-of-mass energy of 8 TeV at the LHC with the CMS detector, in data corresponding to an integrated luminosity of 18.4 fb(-1). The inclusive cross section is found to be 275.6 +/- 6.1 (stat) +/- 37.8 (syst) +/- 7.2 (lumi) pb. The normalized differential cross sections are measured as a function of the top quark transverse momenta, pT, and compared to predictions from quantum chromodynamics....
Show moreThe cross section for tt production in the all-jets final state is measured in pp collisions at a centre-of-mass energy of 8 TeV at the LHC with the CMS detector, in data corresponding to an integrated luminosity of 18.4 fb(-1). The inclusive cross section is found to be 275.6 +/- 6.1 (stat) +/- 37.8 (syst) +/- 7.2 (lumi) pb. The normalized differential cross sections are measured as a function of the top quark transverse momenta, pT, and compared to predictions from quantum chromodynamics. The results are reported at detector, parton, and particle levels. In all cases, the measured top quark pT spectra are significantly softer than theoretical predictions.
Show less - Date Issued
- 2016-03-08
- Identifier
- FSU_libsubv1_wos_000375300800001, 10.1140/epjc/s10052-016-3956-5
- Format
- Citation
- Title
- Interlayer Electronic Transport In Camnbi2 Antiferromagnet.
- Creator
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Wang, Aifeng, Graf, D., Wu, Lijun, Wang, Kefeng, Bozin, E., Zhu, Yimei, Petrovic, C.
- Abstract/Description
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We report interlayer electronic transport in CaMnBi2 single crystals. Quantum oscillations and angular magnetoresistance suggest coherent electronic conduction and valley polarized conduction of Dirac states. The small cyclotron mass, high mobility of carriers, and nontrivial Berry's phase are consistent with the presence of Dirac fermions on the side wall of the warped cylindrical Fermi surface. Similarly to SrMnBi2, which features an anisotropic Dirac cone, our results suggest that magnetic...
Show moreWe report interlayer electronic transport in CaMnBi2 single crystals. Quantum oscillations and angular magnetoresistance suggest coherent electronic conduction and valley polarized conduction of Dirac states. The small cyclotron mass, high mobility of carriers, and nontrivial Berry's phase are consistent with the presence of Dirac fermions on the side wall of the warped cylindrical Fermi surface. Similarly to SrMnBi2, which features an anisotropic Dirac cone, our results suggest that magnetic-field-induced changes in interlayer conduction are also present in layered bismuth-based materials with a zero-energy line in momentum space created by the staggered alkaline earth atoms.
Show less - Date Issued
- 2016-09-12
- Identifier
- FSU_libsubv1_wos_000383145300004, 10.1103/PhysRevB.94.125118
- Format
- Citation
- Title
- Interaction-driven Fractional Quantum Hall State Of Hard-core Bosons On Kagome Lattice At One-third Filling.
- Creator
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Zhu, W., Gong, S. S., Sheng, D. N.
- Abstract/Description
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There has been a growing interest in realizing topologically nontrivial states of matter in band insulators, where a quantum Hall effect can appear as an intrinsic property of the band structure. While ongoing progress is under way with a number of directions, the possibility of realizing novel interaction-generated topological phases, without the requirement of a nontrivial invariant encoded in single-particle wave function or band structure, can significantly extend the class of topological...
Show moreThere has been a growing interest in realizing topologically nontrivial states of matter in band insulators, where a quantum Hall effect can appear as an intrinsic property of the band structure. While ongoing progress is under way with a number of directions, the possibility of realizing novel interaction-generated topological phases, without the requirement of a nontrivial invariant encoded in single-particle wave function or band structure, can significantly extend the class of topological materials and is thus of great importance. Here, we show an interaction-driven topological phase emerging in an extended Bose-Hubbard model on a kagome lattice, where the noninteracting band structure is topological trivial with zero Berry curvature in the Brillouin zone. By means of an unbiased state-of-the-art density-matrix renormalization group technique, we identify that the ground state in a broad parameter region is equivalent to a bosonic fractional quantum Hall Laughlin state, based on the characterization of universal properties including ground-state degeneracy, edge excitations, and anyonic quasiparticle statistics. Our work paves a way to finding an interaction-induced topological phase at the phase boundary of conventionally ordered solid phases.
Show less - Date Issued
- 2016-07-13
- Identifier
- FSU_libsubv1_wos_000379502800001, 10.1103/PhysRevB.94.035129
- Format
- Citation